研究目的
To solve analytically coherent anti‐Stokes Raman scattering (CARS) under asymmetric conditions of chirped femtosecond laser pulses.
研究成果
The analytical model of CARS realized by means of three nonlinearly chirped asymmetric laser pulses is successfully developed, avoiding numerical integration. The model is applied to nitrogen CARS for thermometric reasons, showing good agreement with experimental spectra under different chirp conditions.
研究不足
The model is limited to field phases with cubic frequency dependence and requires approximations to guarantee the solution to the CARS problem under asymmetric conditions.