研究目的
To achieve high-efficiency blade-coated organic solar cells (OSCs) by suppressing the excessive aggregation of non-fullerene acceptor using polymer additive N2200.
研究成果
The addition of N2200 effectively suppresses the excessive aggregation of non-fullerene acceptors in blade-coated OSCs, leading to improved device performance. Large-area devices (1.0 cm2) achieved high efficiencies, demonstrating the potential for scalable production of high-performance OSCs.
研究不足
The study focuses on specific blends of materials (PM6:IT-4F and PM6:Y6) and the effect of N2200 additive. The applicability to other material systems and the long-term stability of the devices were not extensively explored.
1:Experimental Design and Method Selection
The study involved the fabrication of OSCs using blade-coating and spin-coating methods, with the addition of N2200 to suppress the aggregation of non-fullerene acceptors.
2:Sample Selection and Data Sources
Active layers were prepared using blends of PM6:IT-4F and PM6:Y6, with and without the addition of N2200.
3:List of Experimental Equipment and Materials
ITO-coated glass substrates, PEDOT:PSS, PM6, IT-4F, Y6, N2200, PNDIT-F3N, Ag.
4:Experimental Procedures and Operational Workflow
Substrates were cleaned and treated with plasma before coating with PEDOT:PSS. Active layer solutions were prepared and coated using spin-coating or blade-coating methods. Devices were completed with the evaporation of Ag electrodes.
5:Data Analysis Methods
Photovoltaic performance was characterized using J–V curves and EQE measurements. Morphology was investigated using AFM, TEM, XRD, and GIWAXS.
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