研究目的
To investigate the potential of few-layer GeSe for applications in high stability, very fast and broadband optoelectronic devices by fabricating field-effect transistors (FETs) made of few-layer GeSe with direct bandgaps and characterizing their optoelectronic properties.
研究成果
Few-layer GeSe FETs show response to the illumination wavelengths from the visible up to 1400 nm, and rise (fall) time of 13μs (19μs), demonstrating very broadband and fast photodetections. Our results demonstrate the potential of few-layer GeSe for applications in high stability, very fast and broadband of photoresponse nanoelectronic devices and circuitries.
研究不足
The present few-layer GeSe shows a several nanometers of RMS roughness, which may severely decrease the photoresponse speed, and further improve the layer-thinning methods are expected for better performances of the few-layer GeSe FETs.
1:Experimental Design and Method Selection:
Few-layer GeSe FETs are fabricated using mechanical exfoliation, standard FET fabrication, and subsequent focused laser-scan thinning methods.
2:Sample Selection and Data Sources:
GeSe monocrystalline with 3~5 mm sizes and ~
3:3 mm thickness, and 9995% of purity is used as the source material. List of Experimental Equipment and Materials:
A home-made laser scanning confocal microscope is used to thin the GeSe flakes. Au/Ge (90 nm/10 nm) electrodes are fabricated by direct laser lithography.
4:Experimental Procedures and Operational Workflow:
GeSe flakes are transferred to a clean oxidized silicon surface with the SiO2 thickness of 100 nm by mechanical exfoliation. Laser thinned GeSe device with direct bandgaps are schematically shown.
5:Data Analysis Methods:
The field-effect mobility of the few-layer GeSe device is estimated from the linear region based on the equation provided.
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charge coupled device
Andor iDus 416 series
Andor
Measurement of fluorescence spectrum
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CCD
Andor idus InGaAs
Andor
Measurement of fluorescence spectrum in the infrared
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Keithley semiconductor analyzer
SCS4200
Keithley
Electric characterization of the device
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high performance graphics sampling multimeter
Keithley DMM7510
Keithley
Measurement of the photoswitching behavior of the few-layer GeSe FET device
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fluorescence microscope
Olympus BX63
Olympus
Measurement of fluorescence emitted from laser-thinned GeSe nanosheets
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GeSe monocrystalline
2D Semiconductors, Inc. U.S.
Source material for fabricating few-layer GeSe FETs
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laser scanning confocal microscope
Used to thin the GeSe flakes
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Au/Ge electrodes
90 nm/10 nm
Electrodes for the FETs
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spectrometer
Shamrock 303i
Measurement of fluorescence spectrum
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