研究目的
To control the line shape of Fano-like resonances in all-dielectric multilayer structures using UV light irradiation and to investigate the enhanced photochromic response in these structures.
研究成果
The study successfully demonstrated the wide-range control of Fano-like resonances in all-dielectric multilayer structures using UV light irradiation, with the line shape changing from electromagnetically induced transparency-like to electromagnetically induced absorption-like. The enhanced photochromic response in the multilayer structure was attributed to the enhanced local electric fields inside the photochromic waveguide layer.
研究不足
The study is limited by the experimental conditions such as the UV irradiation dose and the specific materials used for the waveguide layers. The influence of thermal backconversion of merocyanine molecules to spiropyran on the observed ATR spectra cannot be completely neglected.
1:Experimental Design and Method Selection:
The study used multilayer structures consisting of a waveguide layer supporting a half-leaky guided mode, a spacer layer, and another waveguide layer supporting a planar waveguide mode. The line shape of Fano-like resonances was controlled by UV light irradiation.
2:Sample Selection and Data Sources:
Two types of samples were prepared, incorporating photochromic and absorptive layers as waveguide layers.
3:List of Experimental Equipment and Materials:
A UV-visible spectrophotometer, UV-LED, He–Ne laser, and spin coating method were used for sample preparation and measurements.
4:Experimental Procedures and Operational Workflow:
Angle-scan ATR measurements were performed before and after UV irradiation, with the dose varied to observe changes in the line shape.
5:Data Analysis Methods:
Electromagnetic calculations and fitting procedures were used to analyze the observed changes in the ATR spectra.
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