研究目的
Investigating the effects of structure and laser gauge choices on the high-harmonic generation process in solids using semiconductor Bloch equations.
研究成果
The study concludes that length-gauge SBEs are computationally more efficient when dephasing and separation of currents are required, while velocity-gauge SBEs are more efficient when only the total current is needed. The inclusion of Berry connections and TDPs is crucial for accurate simulations in systems without inversion or time-reversal symmetries.
研究不足
The study is limited to topologically trivial systems and does not address degenerate manifolds of energy bands. The computational complexity increases with the inclusion of dephasing and separation of currents.
1:Experimental Design and Method Selection:
The study employs semiconductor Bloch equations (SBEs) for simulations of strong-field laser-matter interactions in condensed matter, focusing on systems without inversion or time-reversal symmetries. The methodology includes the construction of a smooth and periodic structure gauge for Bloch states and the investigation of SBEs in length and velocity gauges.
2:Sample Selection and Data Sources:
Two systems are used as numerical examples: a one-dimensional model of ZnO and the two-dimensional monolayer hexagonal boron nitride (hBN).
3:List of Experimental Equipment and Materials:
The study utilizes theoretical models and computational methods without specific physical equipment.
4:Experimental Procedures and Operational Workflow:
The procedure involves solving the time-independent Schr?dinger equation to find Bloch band energies and functions, constructing a relevant structure gauge, and solving the SBEs in the desired laser gauge.
5:Data Analysis Methods:
The analysis includes comparing the computational efficiency and accuracy of SBEs in different gauges and the impact of omitting Berry connections or TDPs on HHG spectra.
独家科研数据包,助您复现前沿成果,加速创新突破
获取完整内容