研究目的
Investigating the strong coupling between localized surface plasmon resonance (LSPR) and surface plasmon polariton (SPP) Bloch wave to manipulate the dephasing time of plasmon modes.
研究成果
The study demonstrates strong coupling between LSPR and SPP-Bloch wave, leading to the manipulation of dephasing time. Near-field measurements in both frequency and time domains provide insights into the coupling extent and dynamic processes. These findings enhance the understanding of plasmonic strong coupling systems and their applications.
研究不足
The study focuses on specific nanostructures and coupling conditions, which may limit the generalizability of the findings to other plasmonic systems. The experimental setup requires precise control over fabrication and measurement conditions.
1:Experimental Design and Method Selection:
The study employs multilayer nanostructures to realize strong coupling between LSPR and SPP-Bloch wave. Far-field and near-field properties are investigated using photoemission electron microscopy (PEEM) in both frequency and time domains.
2:Sample Selection and Data Sources:
Samples are fabricated with gold square nanoblock arrays on an Al2O3 spacer deposited on an ITO-coated glass substrate. Far-field spectral properties are analyzed using a spectrophotometer coupled with a transmission microscope.
3:List of Experimental Equipment and Materials:
Includes a wavelength tunable laser source, PEEM system, spectrophotometer (PMA-11, Hamamatsu), transmission microscope (BX51, Olympus), and FDTD solutions software package for numerical simulation.
4:Experimental Procedures and Operational Workflow:
Fabrication involves EBL and metal evaporation techniques. Near-field and far-field measurements are conducted to observe the coupling effects and dephasing times.
5:Data Analysis Methods:
The dynamic process is analyzed using time-resolved PEEM, and the dephasing time is extracted by fitting the PE signal.
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