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Preparation and characterization of graphene – TiO2 nanocomposite for enhanced photodegradation of Rhodamine-B dye

DOI:10.1016/j.ejar.2018.11.009 期刊:The Egyptian Journal of Aquatic Research 出版年份:2018 更新时间:2025-09-10 09:29:36
摘要: The synthesizing of TiO2@rGO nanocomposites using an efficient method has been carried out to enhance the photodegradation activities of TiO2. Reduced graphene oxide (rGO) synthesis has been illustrated as a key step. The preparation of TiO2@rGO is highly needed and recommended to develop an effective way for the reduction of GO. Our study illustrated an environmentally simple method for TiO2@rGO preparation and demonstrated its efficiency for photocatalytic process by utilizing rhodamine-B dye as an organic pollutant. Synthesized nanoparticles of reduced TiO2@rGO have an observable increase in photo-energy adsorption leading to the increase of the photodegradation reactions. From the obtained results, TiO2@rGO nanocomposites showed great ability to absorb photo-energy and enhance the photodegradation reactions. Moreover, the results revealed that the 3% TiO2@rGO have the best performance than 1% TiO2@rGO at pH = 9.0, 30 mg/l initial dye concentration and 60 min irradiation duration. The reduced graphene oxide production was considered as an influential co-catalyst for improving the TiO2 photocatalytic activities mainly owing to; the fast separation of h+/e? and the adsorption improvement. Our study affirms the production of promising applicable particles using the environmental photocatalysis process in particular with regard to wastewater purification.
作者: Mohamed H.H. Ali,Afify D. Al-Afify,Mohamed E. Goher
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To synthesize TiO2@rGO nanocomposites by an environmentally friendly and easy method and to demonstrate the factors that affect the photodegradation process using rhodamine-B (Rh-B) as the target organic pollutant.

The synthesized TiO2@rGO nanocomposites showed enhanced photocatalytic and degradation activities for eliminating Rh-B dye under certain conditions. The addition of rGO oxide was found to be an efficient catalyst for improving the TiO2 photocatalytic performance. The prepared nanocomposites are promising for applications in environmental photocatalysis, especially in wastewater purification.

The study focused on the photodegradation of Rh-B dye under specific conditions (pH, initial dye concentration, catalyst dose, and irradiation time). The applicability of the synthesized nanocomposites to other pollutants or under different environmental conditions was not explored.

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