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Characterization of time-resolved emission of N<sub>2</sub>(C) in an atmospheric pressure nanosecond pulsed air-plasma using streak spectroscopy

DOI:10.1088/1361-6595/aaf8d3 期刊:Plasma Sources Science and Technology 出版年份:2018 更新时间:2025-09-04 15:30:14
摘要: A new optical emission spectroscopy (OES) system using a streak camera (streak-OES) is developed to obtain highly time-resolved OES measurements of nanosecond-duration pulsed air-plasmas at atmospheric pressure. The newly developed system is used to measure the time evolution of the emission of N2(C), a critical species in the two-step mechanism of rapid heating characteristic of nanosecond pulsed discharges. Time resolution of less than 400 ps is achieved in the current system, a significant improvement over conventional OES measurements with ICCD cameras or photomultiplier tubes (PMTs). In addition, as long as the driving voltage pulse lies within the streak camera sweep window, the entire plasma emission spectrum for a single discharge is acquired. This capability is in contrast to prior studies where the time-dependent emission is obtained by plotting measurements at single steps from separate discharges. The effect of pulse repetition frequency (PRF) on the N2(C) decay is investigated by recording emission spectra for single discharges at 5-100 kHz. The streak images clearly show that the decay time of the N2(C-B,0-0) transition increases as the PRF is increased. The emission decay exhibits two distinct phases with significantly different decay rates, consistent with prior measurements. The 1/e lifetimes of the two decay regimes are found using exponential fits to the emission decay curves. In addition, joint statistics relating the decay times and energy deposited in the plasma were also obtained.
作者: R. Jagannath,A. Satija,R. P. Lucht,S. Bane
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To develop a new optical emission spectroscopy (OES) system using a streak camera (streak-OES) for highly time-resolved OES measurements of nanosecond-duration pulsed air-plasmas at atmospheric pressure and to investigate the effect of pulse repetition frequency (PRF) on the N2(C) decay.

The streak-OES system successfully captured the time-resolved decay profile of N2(C) for single nanosecond-duration spark discharges with a time resolution of less than 400 ps. The study provided joint statistics relating decay times and energy deposited in the plasma, offering insights into the effect of PRF on N2(C) decay. Future work aims to extend the system's capabilities to other species and plasma environments.

The study was limited to atmospheric pressure air-plasmas and focused on the N2(C) emission. The temporal resolution, while significantly improved, was still limited to less than 400 ps. The variability in discharge characteristics due to jitter in the NRP power supply and other factors was noted.

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