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Performance-Enhancing Selector via Symmetrical Multilayer Design

DOI:10.1002/adfm.201808376 期刊:Advanced Functional Materials 出版年份:2019 更新时间:2025-09-23 15:23:52
摘要: Two-terminal selectors with high nonlinearity, based on bidirectional threshold switching (TS) behaviors, are considered as a crucial element of crossbar integration for emerging nonvolatile memory and neuromorphic network. Although great efforts have been made to obtain various selectors, existing selectors cannot fully satisfy the rigorous standard of assorted memristive elements and it is in great demand to enhance the performance. Here, a new type of Ag/TaOx/TaOy/TaOx/Ag (x < y) selector based on homogeneous trilayered oxides is developed to attain the required parameters including bidirectional TS operation, a large selectivity of ≈1010, a high compliance current up to 1 mA, and ultralow switching voltages under 0.2 V. Tunable operation voltages can be realized by modulating the thickness of inserted TaOy. All-TaOx-based integrated 1S1R (one selector and one memristor) cells, prepared completely by magnetron sputtering and no need of a middle electrode, exhibit a nonlinear feature, which is quite characteristic for the crossbar devices, avoiding undesired crosstalk current issues. The tantalum-oxide-based homojunctions offer high insulation, low ion mobility, and rich interfaces, which is responsible for the modulation of Ag conductive filaments and corresponding high-performance cation-based selector. These findings might advance practical implementation of two-terminal selectors in emerging memories, especially resistive random access memories.
作者: Yiming Sun,Xiaolong Zhao,Cheng Song,Kun Xu,Yue Xi,Jun Yin,Ziyu Wang,Xiaofeng Zhou,Xianzhe Chen,Guoyi Shi,Hangbing Lv,Qi Liu,Fei Zeng,Xiaoyan Zhong,Huaqiang Wu,Ming Liu,Feng Pan
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To develop a high-performance two-terminal selector with enhanced parameters such as bidirectional threshold switching, large selectivity, high compliance current, and low switching voltages for integration in crossbar arrays for nonvolatile memory and neuromorphic networks.

The developed Ag/TaOx/TaOy/TaOx/Ag selector exhibits superior performance with bidirectional operation, high selectivity, low voltages, and fast switching, enabling effective integration in 1S1R cells for crossbar arrays without a middle electrode, advancing applications in nonvolatile memory and neuromorphic computing.

The study is limited to tantalum oxide-based materials and specific device structures; scalability to other materials or larger arrays may require further optimization. The experimental conditions are at room temperature and ambient atmosphere, which might not cover all operational environments.

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