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Universal renormalization group flow toward perfect Fermi-surface nesting driven by enhanced electron-electron correlations in monolayer vanadium diselenide

DOI:10.1103/PhysRevB.99.014106 期刊:Physical Review B 出版年份:2019 更新时间:2025-09-23 15:23:52
摘要: Reducing the thickness of three-dimensional samples on appropriate substrates is a promising way to control electron-electron interactions, responsible for so called electronic reconstruction phenomena. Although the electronic reconstruction has been investigated both extensively and intensively in oxide heterostructure interfaces, this paradigm is not well established in the van der Waals heterointerface system. In the present study, we examine the nature of a charge ordering transition in monolayer vanadium diselenide (VSe2). This two-dimensional phase transition would be distinguished from that of VSe2 bulk samples, driven by more enhanced electron-electron correlations. We recall that VSe2 bulk samples show a charge-density-wave (CDW) transition around TCDW ~ 105 K. This bulk phase transition results from Fermi-surface nesting properties, where the low-temperature CDW state coexists with itinerant electrons of residual Fermi surfaces. Recently, angle-resolved photoemission spectroscopy measurements [Nano Lett. 18, 5432 (2018)] uncovered that the Fermi-surface nesting becomes perfect, where the dynamics of hot electrons is dispersionless along the orthogonal direction of the nesting wave vector. In addition, scanning tunneling microscopy measurements [Nano Lett. 18, 5432 (2018)] confirmed that the resulting CDW state shows essentially the same modulation pattern as the three-dimensional system of VSe2. Here, we perform the renormalization group analysis based on an effective-field theory in terms of critical CDW fluctuations and hot electrons of imperfect Fermi-surface nesting. As a result, we reveal that the imperfect nesting universally flows into perfect nesting in two dimensions, where the Fermi velocity along the orthogonal direction of the nesting vector vanishes generically. We argue that this electronic reconstruction is responsible for the observation [Nano Lett. 18, 5432 (2018).] that the CDW transition temperature is much more enhanced to be around TCDW ~ 350 K than that of the bulk sample.
作者: Iksu Jang,Ganbat Duvjir,Byoung Ki Choi,Jungdae Kim,Young Jun Chang,Ki-Seok Kim
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Investigating the universal renormalization group flow toward perfect Fermi-surface nesting driven by enhanced electron-electron correlations in monolayer vanadium diselenide.

The renormalization group analysis reveals that imperfect Fermi-surface nesting universally flows into perfect nesting in two dimensions due to enhanced electron-electron correlations, leading to a drastic increase in the CDW transition temperature in monolayer VSe2 compared to the bulk. This electronic reconstruction is a key mechanism for the observed phenomena, with implications for understanding strongly correlated systems in low dimensions.

The study is theoretical and relies on approximations such as the one-loop renormalization group analysis and dimensional regularization. It does not account for higher-order quantum corrections or disorder effects, and the applicability to real materials may be limited by simplifications in the effective-field theory.

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