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Influence of the capping layer material on the interfacial Dzyaloshinskii-Moriya interaction in Pt/Co/capping layer structures probed by Brillouin light scattering<sup></sup>

DOI:10.1088/1361-6463/aafdf5 期刊:Journal of Physics D: Applied Physics 出版年份:2019 更新时间:2025-09-23 15:22:29
摘要: Influence of the capping layer material on the interfacial Dzyaloshinskii-Moriya interaction in Pt/Co/capping layer structures probed by Brillouin light scattering. Co ultrathin films, of various thicknesses (0.8 nm ≤ tCo ≤ 2.5 nm), have been grown by sputtering on Si substrates, using Pt buffer layers and different capping layers (Cu, Ir, MgO and Pt). The x-ray diffraction revealed that our films have a (111) out-of-plane texture with various degrees of strains. Their magnetic properties have been studied by vibrating sample magnetometry (VSM) and Brillouin light scattering (BLS) in the Damon-Eshbach geometry. VSM characterizations revealed that films with Co thickness below (above) the spin reorientation transition thickness, which is capping layer dependent, are perpendicularly (in-plane) magnetized, suggesting the existence of an interface anisotropy. The magnetic dead layer has been taken into account to precisely determine the surface anisotropy constant was found to be 1.42 ± 0.02 erg/cm2 and of 1.33 ± 0.02 erg/cm2 for the Pt/Co/Cu and Pt/Co/Ir samples, respectively, suggesting that it is due to the Pt/Co interface and that the top Co/Cu or Co/Ir interfaces have a negligible contribution. A lower value of 1.07 ± 0.02 erg/cm2 has been obtained for Pt/Co/MgO most probably due to over-oxidation of Co at the Co/MgO interface. The BLS measurements revealed a pronounced nonreciprocal spin waves propagation, due to the interfacial Dzyaloshinskii-Moriya interaction (iDMI) induced by Pt interface with Co, which increases with decreasing Co thickness. The surface iDMI constant Ds estimated at -0.8 pJ/m, -1.05 pJ/m and –0.95 pJ/m, respectively for Pt/Co/Ir, Pt/Co/Cu and Pt/Co/MgO for the samples where a linear thickness dependence of the effective iDMI constant has been observed.
作者: Mohamed Belmeguenai,Y. Roussigné,S. M. Chérif,A. Stashkevich,T. Petrisor jr.,M. Nasui,M.S. Gabor
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To investigate the influence of capping layer material on the interfacial Dzyaloshinskii-Moriya interaction (iDMI) and interface perpendicular anisotropy in Pt/Co/X multilayers with X = Cu, Ir, MgO, Pt.

The iDMI is mainly induced by the Pt/Co interface, with capping layers (Cu, MgO) having negligible contribution, while Ir reduces iDMI due to interface quality issues. For symmetric Pt/Co/Pt, iDMI cancels out. Surface anisotropy constants are similar for Cu and Ir cappings but lower for MgO due to oxidation. BLS is effective for iDMI characterization, but linear model deviations occur for thin films.

Deviation from linear behavior in iDMI and anisotropy for thinner Co layers due to interface degradation, strain misfit, and decreased Curie temperature; lesser quality of Pt/Co/Ir system affects measurements; iDMI is sample deposition condition dependent.

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