摘要： We developed a facile method for fabricating large-area two-dimensional (2D) organic highly crystalline films and extended it to organic thin-film transistor arrays. Tilted spinning provided oriented flow at the three-phase contact line and 2D crystalline film that consisted of layer-by-layer stacked 2,7-diocty[1]benzothieno[3,2-b]benzothiophene (C8-BTBT) was obtained facilely for organic thin-film transistor (OTFT). The extracted field-effect mobility is 4.6 cm-2 V-1 s-1 but with non-ideal features. By applying this method to microdroplet arrays, oriented crystal was fabricated, and the channel region for OTFTs was covered by adjusting the spinning speed. By tuning the tilt angle (θ) of the revolving substrate, we fabricated high-performance OTFT arrays with average and maximum mobilities of 7.5 and 10.1 cm-2 V-1 s-1, respectively, that exhibited high reliability factors of over 90 % and were closed to ideal transistors. These results suggest that high-quality crystalline film can be obtained via a facile tilted spinning method.