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Wintertime Local Wind Dynamics from Scanning Doppler Lidar and Air Quality in the Arve River Valley
摘要： Air quality issues are frequent in urbanized valleys, particularly in wintertime when a temperature inversion forms and the air within the valley is stably stratified over several days. In addition to pollutant sources, local winds can have a significant impact on the spatial distribution and temporal evolution of pollutant concentrations. They can be very complex and difficult to represent in numerical weather prediction models, particularly under stable conditions. Better knowledge of these local winds from observations is also a prerequisite to improving air quality prediction capability. This paper analyses local winds during the Passy-2015 field experiment that took place in a section of the Arve river valley, near Chamonix–Mont-Blanc. This location is one of the worst places in France regarding air quality. The wind analysis, which is mainly based on scanning Doppler lidar data sampling a persistent temperature inversion episode, reveals features consistent with the higher pollutant concentrations observed in this section of the valley as well as their spatial heterogeneities. In particular, an elevated down-valley jet is observed at night in the northern half of the valley, which, combined with a weak daytime up-valley wind, leads to very poor ventilation of the lowest layers. A northeast–southwest gradient in ventilation is observed on a daily-average, and is consistent with the PM10 heterogeneities observed within the valley.
关键词： scanning Doppler wind lidar,Passy-2015 field experiment,cold air pool,local wind dynamics,air quality,alpine valley
更新于2025-09-23 15:23:52
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Rapid and sensitive detection of formaldehyde using portable 2-dimensional gas chromatography equipped with photoionization detectors
摘要： We developed an automated and highly portable device for rapid and sensitive formaldehyde detection based on heart-cutting 2-dimensional gas chromatography. In this design, the air sample was first absorbed by a preconcentrator before it is injected into the 1st-dimensional column (Rtx?-VMS). The partial elution from the 1st-dimensional column containing formaldehyde was re-injected into the 2nd-dimensional column (Rt? Q-BOND column) for further separation. The detection of formaldehyde was achieved by using a micro-helium dielectric barrier discharge photoionization detector that is able to ionize formaldehyde (ionization potential = 10.88 eV). Due to the use of many miniaturized components, the entire system has a weight of only 1.3 kg (excluding the helium cartridge) and dimensions of only 27 cm x 24 cm x 12 cm. It is capable of detecting formaldehyde down to 0.5 ppb (V/V) with a signal-to-noise ratio of 6 in only 11 min (including 6 min of sampling). Meanwhile, simultaneous separation and detection of other air pollution related toxic compounds, such as benzene, toluene, ethylbenzene, and xylene, was also demonstrated by the 1-dimensional column and a flow-through micro-photoionization detector. The device developed here should have a broad range of applications in environmental protection, industries, space exploration, and battlefield.
关键词： Gas chromatography,Air quality control,Indoor air analysis,Photoionization detector,2D GC,Formaldehyde detection
更新于2025-09-23 15:23:52
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[IEEE IGARSS 2018 - 2018 IEEE International Geoscience and Remote Sensing Symposium - Valencia (2018.7.22-2018.7.27)] IGARSS 2018 - 2018 IEEE International Geoscience and Remote Sensing Symposium - Assessment of Satellite Aerosol Optical Depth to Estimate Particulate Matter Distribution in Valencia City
摘要： The estimation of exposure to PM10 and PM2.5 requires the knowledge of surface concentration at high temporal and spatial resolutions. In this paper, the relation between PM10 and PM2.5 ground data and MODIS AOD satellite data has been evaluated to determine the concentration of particulate matter in Valencia, Spain. This was done using data from the Valencian Network of Surveillance and Control of Air Pollution and the scientific data set "Optical Depth Land and Ocean" from MODIS Terra and Aqua with 3km of spatial resolution. The linear regression model for PM10 provided a regression slope of 25.99 μg.m-3 and an interception of 12.07 μg.m-3 (RMSE = 8.61 μg.m-3), while for PM2.5 the slope and interception were 26.87 μg.m-3 and 5.98 μg.m-3 (RMSE = 5.5 μg.m-3).
关键词： Valencia,particulate matter,air quality,AOD,MODIS
更新于2025-09-23 15:22:29
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The AOTF-based NO<sub>2</sub> camera
摘要： The abundance of NO2 in the boundary layer relates to air quality and pollution source monitoring. Observing the spatiotemporal distribution of NO2 above well-delimited (flue gas stacks, volcanoes, ships) or more extended sources (cities) allows for applications such as monitoring emission fluxes or studying the plume dynamic chemistry and its transport. So far, most attempts to map the NO2 field from the ground have been made with visible-light scanning grating spectrometers. Benefiting from a high retrieval accuracy, they only achieve a relatively low spatiotemporal resolution that hampers the detection of dynamic features. We present a new type of passive remote sensing instrument aiming at the measurement of the 2-D distributions of NO2 slant column densities (SCDs) with a high spatiotemporal resolution. The measurement principle has strong similarities with the popular filter-based SO2 camera as it relies on spectral images taken at wavelengths where the molecule absorption cross section is different. Contrary to the SO2 camera, the spectral selection is performed by an acousto-optical tunable filter (AOTF) capable of resolving the target molecule's spectral features. The NO2 camera capabilities are demonstrated by imaging the NO2 abundance in the plume of a coal-fired power plant. During this experiment, the 2-D distribution of the NO2 SCD was retrieved with a temporal resolution of 3 min and a spatial sampling of 50 cm (over a 250 × 250 m2 area). The detection limit was close to 5 × 1016 molecules cm?2, with a maximum detected SCD of 4 × 1017 molecules cm?2. Illustrating the added value of the NO2 camera measurements, the data reveal the dynamics of the NO to NO2 conversion in the early plume with an unprecedent resolution: from its release in the air, and for 100 m upwards, the observed NO2 plume concentration increased at a rate of 0.75–1.25 g s?1. In joint campaigns with SO2 cameras, the NO2 camera could also help in removing the bias introduced by the NO2 interference with the SO2 spectrum.
关键词： NO2,AOTF,plume,remote sensing,air quality,camera,acousto-optical tunable filter
更新于2025-09-23 15:22:29
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Performance of various commercial TiO <sub/>2</sub> in photocatalytic degradation of a mixture of indoor air pollutants: Effect of photocatalyst and operating parameters
摘要： Photocatalytic oxidation (PCO) air cleaners can be installed in air handling units to reduce occupants’ exposure to hazardous gases, boost indoor air quality, and concomitantly lower HVAC energy consumption by lowering the required ventilation rate. In this work, photocatalytic activity of four commercialized titanium dioxide photocatalysts (P25, PC500, UV100, and S5-300A) for treating a mixture of seven prevalent volatile organic compounds (VOCs) were assessed in a continuous flow reactor. The impacts of major experimental factors namely concentration (15-100 ppb), relative humidity level (0-60% at 23?C), and residence time (0.012-0.05 s) on the removal efficiency and by-products generation were examined. Photocatalysts were characterized by X-ray diffraction (XRD), nitrogen adsorption-desorption, Fourier transform infrared (FTIR), and scanning electron microscopy (SEM). UV100 possessed the highest values for total VOC removal efficiency, which could be attributed to its large surface area, high porosity, good crystallinity, and large population of surface hydroxyls. Regarding relative humidity, two dominant trends were found: i) increasing the humidity resulted in lower removal efficiencies, or ii) existence of an optimum humidity level in some cases. The treatment efficiency followed the order: alcohols > ketones > aromatics > alkanes. The main by-products in the gas phase were formaldehyde, acetaldehyde, acetone, and propionaldehyde.
关键词： titanium dioxide,volatile organic compounds,indoor air quality,photocatalytic oxidation,relative humidity,residence time,by-products
更新于2025-09-23 15:22:29
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Optical particulate matter sensors in PM <sub/>2.5</sub> measurements in atmospheric air
摘要： Monitoring systems are needed to obtain information about particulate matter (PM) concentrations and to make such information accessible to the public. Small, low-cost, optical sensors could be used to improve the spatial and temporal resolution of PM data. The paper presents results of collocated comparison of four low-cost PM sensors and TEOM analyser, conducted from 20-08-2017 to 24-12-2017 in Wroc?aw, Poland. Plantower PMS7003 and Nova Fitness SDS011 sensors proved to be the best in terms of precision and were linearly correlated with TEOM data. Alphasense OPC-N2 sensors exhibited only moderate precision and linearity. Winsen ZH03A sensors had low repeatability between units and only one copy demonstrated good operation possibilities. All tested sensors had a bias in relation to PM2.5 concentrations obtained from TEOM.
关键词： air quality monitoring,PM2.5,particulate matter,TEOM,optical sensors
更新于2025-09-23 15:21:01
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An Evaluation of MODIS-Retrieved Aerosol Optical Depth over AERONET Sites in Alaska
摘要： The air quality monitoring network in Alaska is currently limited to ground-based observations in urban areas and national parks, leaving a large proportion of the state unmonitored. The use of Moderate Resolution Imaging Spectroradiometer MODIS aerosol optical depth (AOD) to estimate ground-level particulate pollution concentrations has been successfully demonstrated around the world and could potentially be used in Alaska. In this work, MODIS AOD measurements at 550 nm were validated against AOD derived from two ground-based Aerosol Robotic Network (AERONET) sunphotometers in Alaska, located at Utqiagvik (previously known as Barrow) and Bonanza Creek, to determine if MODIS AOD from the Terra and Aqua satellites could be used to estimate ground-level particulate pollution concentrations. The MODIS AOD was obtained from MODIS collection 6 using the dark target Land and Ocean algorithms from years 2000 to 2014. MODIS data could only be obtained between the months of April and October; therefore, it was only evaluated for those months. Individual and combined Terra and Aqua MODIS data were considered. The results showed that MODIS collection 6 products at 10-km resolution for Terra and Aqua combined are not valid over land but are valid over the ocean. Note that the individual Terra and Aqua MODIS collection 6 AOD products at 10-km resolution are valid over land individually but not when combined. Results also suggest the MODIS collection 6 AOD products at 3-km resolution are valid over land and ocean and perform better over land than the 10-km product. These findings indicate that MODIS collection 6 AOD products can be used quantitatively in air quality applications in Alaska during the summer months.
关键词： Alaska,Aerosol Optical Depth,Moderate Resolution Imaging Spectroradiometer,Aerosol Robotic Network,air quality
更新于2025-09-23 15:21:01
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[IEEE 2019 Workshop on Recent Advances in Photonics (WRAP) - Guwahati, India (2019.12.13-2019.12.14)] 2019 Workshop on Recent Advances in Photonics (WRAP) - Quantum cascade laser-based in situ measurement of atmospheric CO and CO <sub/>2</sub> in Gandhinagar using 1f and 2f wavelength modulation spectroscopy
摘要： We report the design, development and field deployment of a quantum cascade laser-based tunable diode laser spectroscopy (TDLS) system for high-sensitivity measurement of atmospheric CO and CO2. Two distributed-feedback quantum cascade lasers are used to interrogate the rotational-vibrational transitions of CO at 4594.99 nm and CO2 at 4319.30 nm. The mean mole fraction values for CO and CO2 for the measurements made at Gandhinagar from 19-25 July 2019 are 477 ppb and 486 ppm respectively. The detection limit of the system is 3 ppb CO and 45 ppb CO2 for integration time of 17 s and 69 s respectively.
关键词： air quality monitoring,greenhouse gas monitoring,quantum cascade laser,wavelength modulation spectroscopy
更新于2025-09-23 15:19:57
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Effective and Efficient Photo -Based PM2.5 Concentration Estimation
摘要： Air pollution has become a worldwide concerned issue and automatical estimation of air quality can provide a positive guidance to both individual and industrial behaviors. Given that the traditional instrument-based method requires high economic, labor costs on instrument purchase and maintenance, this paper proposes an effective, efficient, and cheap photo-based method for the air quality estimation in the case of particulate matter (PM2.5). The success of the proposed method lies in extracting two categories of features (including the gradient similarity and distribution shape of pixel values in the saturation map) by observing the photo appearances captured under different PM2.5 concentrations. Specifically, the gradient similarity is extracted to measure the structural information loss with the consideration that PM2.5 attenuates the light rays emitted from the objects and accordingly distorts the structures of the formed photo. Meanwhile, the saturation map is fit by the Weibull distribution to quantify the color information loss. By combining two features, a primary PM2.5 concentration estimator is obtained. Next, a nonlinear function is adopted to map the primary one to the real PM2.5 concentration. Sufficient experiments on real data captured by professional PM2.5 instrument demonstrate the effectiveness and efficiency of the proposed method. Specifically, it is highly consistent with real sensor’s measures and requires low implementation time.
关键词： saturation map,Air quality estimation,PM2.5 concentration,photo-based,gradient similarity
更新于2025-09-19 17:15:36
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Comparative study of selected indoor concentration from selective laser sintering process using virgin and recycled polyamide nylon (PA12)
摘要： Additive manufacturing (AM) stands out as one of the promising technologies that have huge potential towards manufacturing industry. The study on additive manufacturing impact on the environment and occupational exposure are attracting growing attention recently. However, most of the researcher focus on desktop and fused deposition modelling type and less attention given to the industrial type of AM. Usually, during the selective laser sintering process, recycle powder will be used again to reduce cost and waste. This article compares the PM 2.5, carbon dioxide (CO2) and total volatile organic compound (TVOC) concentration between virgin and recycles powder using polyamide-nylon (PA12) towards indoor concentration. Four phases of sampling involve during air sampling accordingly to the Industry Code of Practice on Indoor Air Quality 2010 by DOSH Malaysia. It was found that PM 2.5 and CO2 are mainly generated during the pre-printing process. The recycle powder tended to appear higher compared to virgin powder in terms of PM 2.5, and CO2. The peak value of PM 2.5 is 1452 μg/m3 and CO2 is 1218 ppm are obtained during the pre-printing process during 8 hours of sampling. TVOC concentration from recycling powder is slightly higher during the post- printing phase where confirm the influence of the powder cake and PA12 temperature from the printing process. In summary, this work proves that elective laser sintering (SLS) machine operators are exposed to a significant amount of exposure during the SLS printing process. Mitigation strategies and personal protective equipment are suggested to reduce occupational exposure.
关键词： selective laser sintering,occupational exposure,indoor air quality,polyamide-nylon,Additive manufacturing
更新于2025-09-16 10:30:52