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Nonlinear Optics || Ultrafast and Intense-Field Nonlinear Optics
摘要： There is currently great interest in the physics of ultrashort laser pulses. Recent advances have led to the generation of laser pulses with durations of the order of 1 attosecond (Hentschel et al., 2001). Ultrashort pulses can be used to probe the properties of matter on extremely short time scales. Within the context of nonlinear optics, ultrashort laser pulses are of interest for at least two separate reasons. The ?rst reason is that the nature of nonlinear optical interactions is often profoundly modi?ed through the use of ultrashort laser pulses, in part because of the broad spectral bandwidth necessarily associated with such pulses. The next two sections of this chapter treat various aspects of the resulting modi?cations of the nature of nonlinear optical interactions. The second reason is that ultrashort laser pulses tend to possess extremely high peak intensities (because laser pulse energies tend to be established by the energy-storage capabilities of laser gain media), and thus short laser pulses tend to have much higher peak powers than longer pulses. The second half of this chapter is devoted to a survey of the sorts of nonlinear optical processes that can be excited by extremely intense laser ?elds.
关键词： attosecond pulses,ultrashort laser pulses,high peak intensities,spectral bandwidth,nonlinear optics
更新于2025-09-23 15:21:01
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Giant Isolated Attosecond Pulses from Two-Color Laser-Plasma Interactions
摘要： A new regime in the interaction of a two-color (ω; 2ω) laser with a nanometer-scale foil is identified, resulting in the emission of extremely intense, isolated attosecond pulses—even in the case of multicycle lasers. For foils irradiated by lasers exceeding the blow-out field strength (i.e., capable of fully separating electrons from the ion background), the addition of a second harmonic field results in the stabilization of the foil up to the blow-out intensity. This is then followed by a sharp transition to transparency that essentially occurs in a single optical cycle. During the transition cycle, a dense, nanometer-scale electron bunch is accelerated to relativistic velocities and emits a single, strong attosecond pulse with a peak intensity approaching that of the laser field.
关键词： two-color laser,laser-plasma interactions,attosecond pulses,coherent synchrotron emission
更新于2025-09-23 15:19:57
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Attosecond pulse shaping using a seeded free-electron laser
摘要： Attosecond pulses are central to the investigation of valence- and core-electron dynamics on their natural timescales1–3. The reproducible generation and characterization of attosecond waveforms has been demonstrated so far only through the process of high-order harmonic generation4–7. Several methods for shaping attosecond waveforms have been proposed, including the use of metallic filters8,9, multilayer mirrors10 and manipulation of the driving field11. However, none of these approaches allows the flexible manipulation of the temporal characteristics of the attosecond waveforms, and they suffer from the low conversion efficiency of the high-order harmonic generation process. Free-electron lasers, by contrast, deliver femtosecond, extreme-ultraviolet and X-ray pulses with energies ranging from tens of microjoules to a few millijoules12,13. Recent experiments have shown that they can generate subfemtosecond spikes, but with temporal characteristics that change shot-to-shot14–16. Here we report reproducible generation of high-energy (microjoule level) attosecond waveforms using a seeded free-electron laser17. We demonstrate amplitude and phase manipulation of the harmonic components of an attosecond pulse train in combination with an approach for its temporal reconstruction. The results presented here open the way to performing attosecond time-resolved experiments with free-electron lasers.
关键词： high-order harmonic generation,Attosecond pulses,temporal reconstruction,free-electron laser
更新于2025-09-19 17:13:59
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Generation of Neara??Circularly Polarized Attosecond Pulse with Tunable Helicity by Unidirectionally Rotating Laser Field
摘要： A method to produce circularly polarized attosecond pulses with tunable helicity from CO molecule by using an unidirectionally rotating laser field is proposed. It is found that broadband harmonic supercontinuum with circular polarization can be generated from the oriented CO molecule. This enables the production sub-100 attosecond isolated pulse with the ellipticity as high as 0.9 at the macroscopic level. Moreover, the helicity of the generated high-order harmonics and the attosecond pulse can be tuned by adjusting the orientation of the CO molecule. This method will be beneficial for the studies on chiral-specific dynamics and magnetic circular dichroism on an attosecond time scale.
关键词： attosecond pulses,tunable helicity,high-order harmonics,rotating laser fields
更新于2025-09-19 17:13:59
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Intense attosecond pulses carrying orbital angular momentum using laser plasma interactions
摘要： Light beams with helical phase-fronts are known to carry orbital angular momentum (OAM) and provide an additional degree of freedom to beams of coherent light. While OAM beams can be readily derived from Gaussian laser beams with phase plates or gratings, this is far more challenging in the extreme ultra-violet (XUV), especially for the case of high XUV intensity. Here, we theoretically and numerically demonstrate that intense surface harmonics carrying OAM are naturally produced by the intrinsic dynamics of a relativistically intense circularly-polarized Gaussian beam (i.e. non-vortex) interacting with a target at normal incidence. Relativistic surface oscillations convert the laser pulses to intense XUV harmonic radiation via the well-known relativistic oscillating mirror mechanism. We show that the azimuthal and radial dependence of the harmonic generation process converts the spin angular momentum of the laser beam to orbital angular momentum resulting in an intense attosecond pulse (or pulse train) with OAM.
关键词： laser plasma interactions,orbital angular momentum,relativistic oscillating mirror,extreme ultra-violet,attosecond pulses
更新于2025-09-12 10:27:22
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[IEEE 2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) - Munich, Germany (2019.6.23-2019.6.27)] 2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) - High Efficiency, High Energy Few-Cycle Driver at 1-μm
摘要： The recent development of high repetition rate lasers based on ytterbium-doped fiber amplifiers (YDFA), has paved the way to increase the repetition rate (>100 kHz) of coherent extreme ultra violet (XUV) sources generated by high harmonic generation (HHG). High repetition rate HHG driver comes with several advantages, such as increased photon flux [1], reduction of the acquisition time in coincidence experiments to study molecular dynamics such as COLTRIMS, and the possibility to study the electronic structure of matter via photoemission spectroscopy and microscopy, where low doses are needed to avoid space-charge effects [2]. Up to now, the overall majority of HHG studies and applications has been restricted to the low repetition rates of Ti:sapphire lasers. Commonly, Ti:sapphire lasers delivers 20 fs pulses at a central wavelength λ = 800 nm, with pulse energies up to hundreds of mJ. However, the average power of these laser systems cannot easily be scaled beyond 10 W, restricting HHG at low repetition rates (up to 10 kHz). Currently, the most mature and powerful ultrafast source technology is undoubtedly ytterbium-based systems, with average power levels beyond 1 kW [3] and numerous industrial applications. However, the long pulse duration of around >200 fs delivered by YDFA sources limits their relevance to this application field. Therefore, nonlinear compression setups have been used successfully to reduce the pulse duration and obtain XUV photon flux among the highest ever reported for HHG-based sources [1]. However, to reach sub-3 cycles regime (< 10 fs at 1030 nm), which is typically required in combination with gating techniques to obtain isolated attosecond pulses, two stages of compression must usually be implemented [4]. This reduces the energy efficiency of the systems dedicated to attosecond physics to typically less than 30% of the overall YDA energy. Here, we demonstrate a two-cycle-source based on a high-energy femtosecond YDFA followed by a hybrid two-stage nonlinear compression setup. The association of a multipass cell-based stage and large-diameter capillary stage provides a compression factor of 48 with an overall transmission of 61%. This source is, to the best of our knowledge, the most efficient few cycle, high energy and high repetition rate laser demonstrated to date. It is very compact with an overall footprint of 1.8 m × 1.0 m and provides a stable train of few-cycle pulses at a central wavelength of 1030 nm that has been continuously characterized over more than 8h. The delivered 6.8 fs (see Fig. 1) 140 μJ pulses at 150 kHz repetition rate, corresponding to 21 W average power, are ideally suited to drive high-photon flux XUV sources [5] through HHG. The described laser system is robust, compact, and power efficient, making it an ideal driver laser for application-ready high flux XUV and attosecond sources.
关键词： attosecond pulses,high harmonic generation,ytterbium-doped fiber amplifiers,extreme ultra violet,high repetition rate lasers
更新于2025-09-12 10:27:22
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[IEEE 2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) - Munich, Germany (2019.6.23-2019.6.27)] 2019 Conference on Lasers and Electro-Optics Europe & European Quantum Electronics Conference (CLEO/Europe-EQEC) - Interferometric Attosecond Lock-in Measurement of Extreme Ultraviolet Circular Diehroism
摘要： Probing vectorial properties of light-matter interactions requires control over the polarization state of light. The generation of extreme-ultraviolet (XUV) attosecond pulses opened new perspectives in measurements of chiral phenomena. Recently, new methods for polarization control in the XUV range, which are based on manipulation of the high harmonic generation (HHG) process were demonstrated [1-4]. However, the limited polarization control in this regime prevents the development of advanced measurement schemes for weak vectorial signals, which require polarization modulation. In our work [5], we establish an XUV lock-in detection scheme, allowing the isolation and amplification of extremely weak chiral signals, by achieving a dynamical control over the polarization state of the XUV light. We demonstrate a time-domain approach to control and modulate the polarization state. This scheme enables us to characterize the polarization state via an in-situ measurement (see Figure 1a,d,e). Our approach, resembling a birefringent crystal for the visible range, is based on the collinear superposition of two independent, phase-locked, orthogonally polarized XUV sources and the control of their relative delay with sub-cycle accuracy (see Figure 1b). We achieve lock-in detection of XUV magnetic circular dichroism (XMCD) in cobalt, transferring weak amplitude variations into a phase modulation (see Figure 1c), by controlling the relative angle, θ , between the two linearly polarized sources. This approach holds the potential of significantly extending the scope of vectorial measurements to the attosecond and nanometer frontiers.
关键词： attosecond pulses,polarization control,high harmonic generation,extreme-ultraviolet,chiral signals,XUV magnetic circular dichroism,XUV lock-in detection
更新于2025-09-11 14:15:04
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Symmetry of molecular Rydberg states revealed by XUV transient absorption spectroscopy
摘要： Transient absorption spectroscopy is utilized extensively for measurements of bound- and quasibound-state dynamics of atoms and molecules. The extension of this technique into the extreme ultraviolet (XUV) region with attosecond pulses has the potential to attain unprecedented time resolution. Here we apply this technique to aligned-in-space molecules. The XUV pulses are much shorter than the time during which the molecules remain aligned, typically <100 fs. However, transient absorption is not an instantaneous probe, because long-lived coherences re-emit for picoseconds to nanoseconds. Due to dephasing of the rotational wavepacket, it is not clear if these coherences will be evident in the absorption spectrum, and whether the properties of the initial excitations will be preserved. We studied Rydberg states of N2 and O2 from 12 to 23 eV. We were able to determine the polarization direction of the electronic transitions, and hence identify the symmetry of the final states.
关键词： transient absorption spectroscopy,extreme ultraviolet,attosecond pulses,molecular alignment,Rydberg states
更新于2025-09-11 14:15:04
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Light for brevity
摘要： The shortest time interval controlled by a human being is the duration of a light pulse as short as only 100 attoseconds, i.e., 10-16 s. This “attosecond” light pulse belongs to the extreme ultraviolet range (XUV) of the electromagnetic spectrum, with central photon energy typically between 20 and 200 eV. Related to its brevity, an attosecond pulse has a broad bandwidth covering tens of eV. These are natural time and energy scales to study electron dynamics in atoms and molecules.
关键词： ultrafast atomic and molecular physics,high-order harmonic generation,attosecond pulses,electron dynamics
更新于2025-09-10 09:29:36
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Vortex Dynamics and Optical Vortices || Ultrashort Extreme Ultraviolet Vortices
摘要： Optical vortices are very attractive because they transport a well-defined orbital angular momentum (OAM) associated with the singularity of the beam. These singular beams, commonly generated in the optical regime, are used in a wide range of applications: communication, micromanipulation, microscopy, among others. The production of OAM beams in the extreme ultraviolet (XUV) and X-ray regimes is of great interest as it allows to extend the applications of optical vortices down to the nanometric scale. Several proposals have been explored in order to generate XUV vortices in synchrotrons and FEL facilities. Here, we study the generation of XUV vortices through high-order harmonic generation (HHG). HHG is a unique source of coherent radiation extending from the XUV to the soft X-ray regime, emitted in the form of attosecond pulses. When driving HHG by OAM beams, highly charged XUV vortices with unprecedented spatiotemporal properties are emitted in the form of helical attosecond beams. In this chapter, we revise our theoretical work in the generation of XUV vortices by HHG. In particular, we illustrate in detail the role of macroscopic phase matching of high-order harmonics when driven by OAM beams, which allows to control the production of attosecond beams carrying OAM.
关键词： attosecond helical beams,ultrafast phenomena,orbital angular momentum,attosecond pulses,extreme ultraviolet vortices,high harmonic generation,nonlinear optics,phase matching
更新于2025-09-09 09:28:46