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- 2019
- 2018
- Dual Material Gate (DMG)
- Vertical TFET
- Single Material Gate(SMG)
- Band-to-band tunneling (BTBT)
- characterization
- organic light-emitting diode
- mobility
- material parameter
- doping
- Electronic Science and Technology
- Optoelectronic Information Science and Engineering
- Fluxim AG
- Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP) and Institute for Applied Physics, Technische Universit?t Dresden
- National Institute of Technology Silchar
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Facile synthesis of a??lucky clovera?? hole-transport material for efficient and stable large-area perovskite solar cells
摘要： Hole-transporting materials (HTMs) play a vital role of transporting holes from the perovskite layer to the counter electrode in perovskite solar cells (PSCs). A novel HTM BTPA-8 is feasibly synthesized by incorporating four dimethoxytriphenylamine leaflets and anthracene-based central bridge. BTPA-8 exhibits a suitable band alignment with MAPbI3 (MA ? CH3NH3) or FA0.85MA0.15PbI3 (FA?HC(NH2)2), high hole mobility, and high thermal stability. The best FA0.85MA0.15PbI3 device based on BTPA-8 exhibits a power conversion efficiency (PCE) of 17.99% in the reverse scan with an aperture area of 0.09 cm2. Under the same condition, a PCE of 18.92% is achieved by the solar cell based on the standard spiro-OMeTAD (2,2,7,7-tetrakis-(N,N-di-p-methoxyphenylamine)-9,9-spirobifluorene). A comparable PCE of 12.31% is also obtained for BTPA-8 based MAPbI3 device compared with spiro-OMeTAD (13.25%) with an aperture area >1 cm2. BTPA-8 based PSCs exhibit better long-term stability than spiro-OMeTAD due to its high hydrophobicity. A lower synthesis cost of BTPA-8 than that of spiro-OMeTAD along with the elevated long-term stability makes it promising for application in PSCs.
关键词： Perovskite solar cells,Hole-transporting material,Anthracene,Low cost
更新于2025-09-23 15:21:01
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Late-stage Customization in Volume Production of Organic Photovoltaics
摘要： Organic photovoltaics (OPV) in free-form shapes have become a unique feature compared to other thin-film photovoltaic technologies. The ability to conform coated layers to any form of shape or structure is a game changer for OPV and creates a paradigm shift in conventional energy businesses. As urban growth prevails, the energy requirement must be compensated by modern means and OPVs provide unique properties where its form or shape can be fully customized. This creates a synergy as they are then easily integrated onto structures or even products. By doing so not only the space requirements are diminished but the energy is delivered directly to the point of use rather than having them transported from central harvesting. The present communication discusses the advances in realizing such free-from patterns by structuring the functional layers to shape after they have been deposited which is referred to as late-stage customization. Using this approach, a pre-coated generic OPV material can be converted into any design upon customer request. The advantages include easier planning, shorter lead times in production as well as paving the way towards lean manufacturing.
关键词： renewable energies,mass production,organic photovoltaics (OPV),laser scribing,slot-die coating,module customization,roll-to-roll fabrication,dielectric material
更新于2025-09-23 15:21:01
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Generating Silicon Nanofiber Clusters from Grinding Sludge by Millisecond Pulsed Laser Irradiation
摘要： Silicon nano?ber clusters were successfully generated by the irradiation of millisecond pulsed laser light on silicon sludge disposed from wafer back-grinding processes. It was found that the size, intensity, and growing speed of the laser-induced plume varied with the gas pressure, while the size and morphology of the nano?bers were dependent on the laser pulse duration. The generated nano?bers were mainly amorphous with crystalline nanoparticles on their tips. The crystallinity and oxidation degree of the nano?bers depended on the preheating conditions of the silicon sludge. This study demonstrated the possibility of changing silicon waste into functional nanomaterials, which are possibly useful for fabricating high-performance lithium-ion battery electrodes.
关键词： laser processing,sludge waste,silicon nano?ber,material reuse,nanostructure
更新于2025-09-23 15:21:01
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New Developments for the Repair of Structural Engine Components with Laser Material Deposition
摘要： Driven by today’s typical “power by the hour” type aftermarket support contracts (e.g. Corporate Care and Total Care) the demands for continuous operation of aircraft engines have increased significantly. For this reason, any disruption caused by heavy maintenance needs to be avoided. Where needed, repair operations should be as time, cost and material efficient as possible. However, service disruptions will still occur and wherever possible, the resulting maintenance intervention activities should take place either “on-wing” or “near-wing”. Consequently, it is the intention of Rolls-Royce to introduce more and more in-situ and minimal invasive maintenance capabilities, such as endoscopic laser material deposition (LMD), for the repair of structural engine components. This article describes the challenges of the minimal invasive LMD process inside cavities and the continued development requirements over and above today’s state-of-the-art repair capability. It also provides further insight concerning the ongoing development of equipment that combines viewing and LMD capability and an outlook on the application of the developed technology.
关键词： Endoscopic Devices,Laser Material Deposition,Structural Engine Components,Rolls-Royce,In-situ Repair
更新于2025-09-23 15:21:01
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Selective laser melting 316L/CuSn10 multi-materials: Processing optimization, interfacial characterization and mechanical property
摘要： Adopting selective laser melting (SLM), a typical technology of additive manufacturing (AM), to form multi-material metallic composites is a challenging and promising field. In this study, SLM 316L/CuSn10 multi-material composites was an innovative attempt to develop functional and structural materials with excellent properties of steel and copper alloys. Dense 316L/CuSn10 specimens with no interfacial macrocracks were successfully fabricated. Results showed that the Vickers microhardness gradually decreased from 329.5±12.5 HV in 316L region to 172.8HV±7.4 in CuSn10 region. The ultimate tensile strength and flexural strength of 316L/CuSn10 sample was 210 MPa, which was higher than the steel/copper alloys fabricated by other methods. It indicated an ideal interfacial bonding condition of 316L/CuSn10 multi-material, which was benefited from sufficient agitation of the molten pools and elements diffusion in the term of continuous distribution of elements and the enrichment of the heterogeneous alloy phases. Also, the grain refinement by re-melting and recrystallization upgraded the bonding performance at the interface. Finally, the 316L/CuSn10 lattice structure was formed by SLM, hinting at the prospects for industrial applications of steel/copper multi-material by SLM in future.
关键词： Selective laser melting (SLM),Mechanical properties,Interface,316L/CuSn10,Multi-material,Microstructure
更新于2025-09-23 15:21:01
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Improved Color Purity of Monolithic Full Color Micro-LEDs Using Distributed Bragg Reflector and Blue Light Absorption Material
摘要： In this study, CdSe/ZnS core-shell quantum dots (QDs) with various dimensions were used as the color conversion materials. QDs with dimensions of 3 nm and 5 nm were excited by gallium nitride (GaN)-based blue micro-light-emitting diodes (micro-LEDs) with a size of 30 μm × 30 μm to respectively form the green and red lights. The hybrid Bragg re?ector (HBR) with high re?ectivity at the regions of the blue, green, and red lights was fabricated on the bottom side of the micro-LEDs to re?ect the downward light. This could enhance the intensity of the green and red lights for the green and red QDs/micro-LEDs to 11% and 10%. The distributed Bragg re?ector (DBR) was fabricated on the QDs color conversion layers to re?ect the non-absorbed blue light that was not absorbed by the QDs, which could increase the probability of the QDs excited by the re?ected blue light. The blue light absorption material was deposited on the DBR to absorb the blue light that escaped from the DBR, which could enhance the color purity of the resulting green and red QDs/micro-LEDs to 90.9% and 90.3%, respectively.
关键词： micro-light-emitting diodes,color conversion layer,distributed Bragg re?ector,quantum dots,hybrid Bragg re?ector,blue light absorption material
更新于2025-09-23 15:21:01
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Structural and Electrical Investigation of Cobalt-Doped NiOx/Perovskite Interface for Efficient Inverted Solar Cells
摘要： Inorganic hole-transporting materials (HTMs) for stable and cheap inverted perovskite-based solar cells are highly desired. In this context, NiOx, with low synthesis temperature, has been employed. However, the low conductivity and the large number of defects limit the boost of the e?ciency. An approach to improve the conductivity is metal doping. In this work, we have synthesized cobalt-doped NiOx nanoparticles containing 0.75, 1, 1.25, 2.5, and 5 mol% cobalt (Co) ions to be used for the inverted planar perovskite solar cells. The best e?ciency of the devices utilizing the low temperature-deposited Co-doped NiOx HTM obtained a champion photoconversion e?ciency of 16.42%, with 0.75 mol% of doping. Interestingly, we demonstrated that the improvement is not from an increase of the conductivity of the NiOx ?lm, but due to the improvement of the perovskite layer morphology. We observe that the Co-doping raises the interfacial recombination of the device but more importantly improves the perovskite morphology, enlarging grain size and reducing the density of bulk defects and the bulk recombination. In the case of 0.75 mol% of doping, the bene?cial e?ects do not just compensate for the deleterious one but increase performance further. Therefore, 0.75 mol% Co doping results in a signi?cant improvement in the performance of NiOx-based inverted planar perovskite solar cells, and represents a good compromise to synthesize, and deposit, the inorganic material at low temperature, without losing the performance, due to the strong impact on the structural properties of the perovskite. This work highlights the importance of the interface from two di?erent points of view, electrical and structural, recognizing the role of a low doping Co concentration, as a key to improve the inverted perovskite-based solar cells’ performance.
关键词： hole transport material,inverted planar perovskite solar cell,perovskite morphology,Co-doped NiOx,electrical conductivity
更新于2025-09-23 15:21:01
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An Experimental and Theoretical Study into Interface Structure and Band Alignment of the Cu2Zn1-xCdxSnS4 Heterointerface for Photovoltaic Applications
摘要： To improve the constraints of kesterite Cu2ZnSnS4 (CZTS) solar cell, such as undesirable band alignment at p?n interfaces, bandgap tuning, and fast carrier recombination, cadmium (Cd) is introduced into CZTS nanocrystals forming Cu2Zn1-xCdxSnS4 through cost-effective solution-based method without post-annealing or sulfurization treatments. A synergetic experimental-theoretical approach was employed to characterize and assess the optoelectronic properties of Cu2Zn1-xCdxSnS4 materials. Tunable direct band gap energy ranging from 1.51 eV to 1.03 eV with high absorption coefficient was demonstrated for the Cu2Zn1-xCdxSnS4 nanocrystals with changing Zn/Cd ratio. Such bandgap engineering in Cu2Zn1-xCdxSnS4 helps in effective carrier separation at interface. Ultrafast spectroscopy reveals a longer lifetime and efficient separation photo-excited charge carriers in Cu2CdSnS4 (CCTS) nanocrystals compared to that of CZTS. We found that there exists a type-II staggered band alignment at the CZTS (CCTS)/CdS interface, from cyclic voltammetric (CV) measurements, corroborated by first-principles density functional theory (DFT) calculations, predicting smaller conduction band offset (CBO) at the CCTS/CdS interface as compared to the CZTS/CdS interface. These results point towards efficient separation of photoexcited carriers across the p?n junction in the ultrafast time scale and highlight a route to improve device performances.
关键词： grain boundary,photovoltaic,cation substitution,Earth-abundant material,interfacial engineering,band offset,ultrafast carrier dynamics
更新于2025-09-23 15:21:01
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2D-SnS$_2$ Nanoflakes Based Efficient Ultraviolet Photodetector
摘要： This paper reports a SnS2 nanoflakes based UV photodetector having high sensitivity and thermal stability upto 120 ?C. Simple and low cost solvothermal technique has been used to synthesize SnS2 nanoflakes of close to hexagonal shapes. A simple photoconductor structure on SiO2/Si substrate is fabricated by using Ag as contact material. The resultant device has good sensitivity (～400), responsivity (～5.5 A/W), EQE (～1868%), detectivity (～1.72 × 1013 Jones) and low response time (～2.2 s). The reported characteristics are superior to many other UV photodetectors utilizing complex hybrid structure of the device, either in form of additional filter layer or nanostructural light sensitive material.
关键词： photoconductor,UV photodetector,SnS2 nanoflakes,2-D material
更新于2025-09-23 15:21:01
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Influence of Electrode Configurations on the Interruption Capacity of Laser Triggered Vacuum Switch
摘要： The electrode configurations have an important effect on the interruption performances of laser triggered vacuum switch (LTVS), but few works pay attention to it so far. The objective of this article is to study the interruption capacity of LTVS with different electrode configurations. The 3-D simulation models of axial magnetic field (AMF) electrode and transverse magnetic field (TMF) electrode are built up, and the magnetic field distributions are calculated and compared. The test platform is set up based on a detachable vacuum chamber. The interruption capacity of LTVS with different electrode structures, electrode spacings, and polarity configurations is studied and analyzed. The test results prove that, compared to the AMF electrode, the interruption capacity of LTVS under the TMF electrode is obviously better, but it is more susceptible to the electrode spacing, and gradually decreases with the increase of electrode spacing. Influence of polarity configuration on the interruption capacity of LTVS is closely related to the target material. The LTVS with KCl + Ti under the positive polarity configuration shows better interruption capacity than negative polarity configuration. The works in this article provide references for the design of LTVS products.
关键词： target material,electrode configurations,laser triggered vacuum switch (LTVS),interruption capacity,Dielectric recovery
更新于2025-09-23 15:21:01