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- 2019
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- Dual Material Gate (DMG)
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- Electronic Science and Technology
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- Fluxim AG
- Dresden Integrated Center for Applied Physics and Photonic Materials (IAPP) and Institute for Applied Physics, Technische Universit?t Dresden
- National Institute of Technology Silchar
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Preparation of graphene oxide with large lateral size and graphene/polyimide hybrid film via in situ “molecular welding” strategy
摘要： In this letter, we report an "ultrasonication-free" direct exfoliation method to obtain graphene oxide with large lateral size (LGO). The average size of LGO sheets is about 50 lm * 50 lm. The g-LGO film shows a superior in-plane thermal conductivity after the graphitization treatment. Furthermore, the in situ "molecular welding", using polyimide (PI) to weld up the GO sheets, is conducted to improve the performance of hybrid thermal conducting film. The thermal conductivity of g-LGO/PI film is 1053.975 ± 8.762 W m-1 K-1, superior to that of the g-LGO film and g-SGO/PI. The direct preparation method to obtain GO with large lateral size, followed by such an in situ "molecular welding" strategy by PI, provides a promising way to fabricate graphene-based film for efficient thermal management.
关键词： Molecular welding,In situ polymerization,Large lateral size,Thermal properties,Carbon material
更新于2025-09-23 15:23:52
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[IEEE 2018 IEEE ISAF-FMA-AMF-AMEC-PFM Joint Conference (IFAAP) - Hiroshima (2018.5.27-2018.6.1)] 2018 IEEE ISAF-FMA-AMF-AMEC-PFM Joint Conference (IFAAP) - Data-Mining Driven Design for Novel Perovskite-type Piezoceramics
摘要： Materials Genome Initiative is envisioning the discovery, development, manufacturing and deployment of advanced materials twice as fast and at a fraction of cost. High throughput computation and experimentation will generate big data, which underscores the emergence of the fourth paradigm---data science. In contrast to machine-learning needing big-data, data-mining assisted by domain knowledge and expertise works well with a limited number of data. In this presentation, data-mining based on material genome approach were performed in field of perovskite-type oxides. New ferroelectric ceramics based on BiFeO3 for high temperature piezoelectric applications are realized with piezoresponse of 1.5~4.0 times the present commercial non-perovskite counterpart. Our essay demonstrates data-mining driven searching sure able to reduce time-to-insight and human effort on synthesization, accelerating new materials discovery and deployment.
关键词： piezoceramics,perovskite-type oxides,material genome approach,high Curie temperature,data-mining
更新于2025-09-23 15:23:52
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The effect of cut depth and distribution for abrasives on wafer surface morphology in diamond wire sawing of PV polycrystalline silicon
摘要： Due to the existence of an acid etch resistant thin amorphous silicon layer over the smooth grooves of the diamond wire sawing polycrystalline silicon wafer surface, the anti-re?ection e?ect is usually not ideal using the mature acidic texturization. The amorphous silicon layer will be produced on the machined surface by material ductile removal. Therefore, during the process of cutting photovoltaic polycrystalline silicon wafers, the material removed in the brittle way is expected and the surface topography of the wafers formed with the brittle fracture is better for the texture fabricating. In this paper, a mathematical model considering the in?uences of process parameters and wire saw parameters was developed based on indentation fracture mechanics. The variations of cutting groove pro?le formed by di?erent material removal modes were also included. The e?ect of abrasives distributed on the wire saw on material removal and surface formation of polysilicon was analyzed. The results showed that most of abrasives removed material with ductile removal mode, however, the volume of the material removed by abrasive in ductile mode is less than 10% of the total removal volume. Brittle fracture removal mode was still the major way of material removal in diamond wire sawing. With the same ratio of the feed rate and wire speed, the faster feed rate and wire speed will not only improve the cutting e?ciency, but also is easier to obtain a brittle fracture surface. There is a critical angle θc for the distribution of abrasives on the wire saw surface. Only when the position angle of the abrasive removing material in brittle mode is less than θc, the brittle fracture can be formed on the wafers surface.
关键词： Diamond wire sawing,Depth of cut,Material removal mode,Photovoltaic polycrystalline silicon
更新于2025-09-23 15:23:52
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Optical memory characteristics of solution-processed organic transistors with self-organized organic floating gates for printable multi-level storage devices
摘要： Exploring optical memory functions in nonvolatile organic field-effect transistor (OFET) memories with top-gate/bottom-contact (TG/BC) configurations can offer effective routes for developing printable, high-density organic memory circuits capable of multi-level data storage. Here, we use a solution process to fabricate TG/BC OFET devices with organic floating-gate structures and investigate their memory characteristics under light illumination. A solution-processable organic composite of 6,13-bis(triisopropylsilylethynyl)pentacene (TIPS-pentacene) and poly(methylmethacrylate) is employed to self-organize organic floating-gate structures on a solution-processed semiconductor layer composed of poly(3-hexylthiophene) (P3HT). The floating-gate OFET devices programmed with blue, green, and red light exhibit large threshold voltage (Vth) shifts of approximately 30 V and stable charge retention characteristics even under light illumination. The devices also exhibit high sensitivity to incident light during programming, and the degree of Vth shift and the on-state current can be tuned using light and programming voltage to facilitate distinct storage and readout of multi-level data.
关键词： floating-gate memory,organic field-effect transistor,top-gate/bottom-contact configuration,multi-level data storage,solution-processable organic material
更新于2025-09-23 15:23:52
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A CSRR-Based Sensor for Full Characterization of Magneto-Dielectric Materials
摘要： In this paper, a novel complementary split-ring resonator (CSRR)-based sensor for full characterization of magneto-dielectric materials is proposed. In general, the operation of microwave resonance-based sensor hinges on the shift in the resonance frequency and the change in the quality factor of the loaded structure. However, both the electric permittivity and the magnetic permeability of the material under test (MUT) have similar effect on the response of the sensor that makes the simultaneous determination of the permittivity and permeability challenging. To remove this difficulty, the main idea behind this paper is to localize the highest intensity of the electric and magnetic fields in two separate zones. By the analysis of the measured resonance frequency and quality factor, the real and imaginary parts of the electric permittivity and the magnetic permeability of the MUT can be determined. Although the characterization of the permittivity and permeability of materials using split-ring resonator and CSRR-based sensors has been widely used, to the best of our knowledge, the full characterization of magneto-dielectric materials using a single sensor has not yet been reported in this paper. As a proof of concept, the sensor was fabricated and used to measure the permittivity and permeability of several materials. Strong agreement between the extracted values and the reference data was achieved.
关键词： sensor,Complementary split ring resonator (CSRR),material characterization,split ring resonator (SRR),magneto-dielectric materials,permittivity and permeability
更新于2025-09-23 15:23:52
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Facile synthesis of two-dimensional tailored graphitic carbon nitride with enhanced photoelectrochemical properties through a three-step polycondensation method for photocatalysis and photoelectrochemical immunosensor
摘要： Graphitic carbon nitride (g-C3N4) is an ideal alternative two-dimensional (2D) nanostructure for photocatalysis and photoelectrochemical (PEC) application, while controllably fabricating 2D shaped g-C3N4 nanolayers/nanosheets is still facing challenges. On the basis of temperature-dependent polymorphic characters, herein, a 2D extending g-C3N4 (g-CNS3) is synthesized from dicyandiamide as the precursor by operating the condensation temperature in a continuously three-step thermal polycondensation procedure. The g-CNS3 with film-like morphology showed improved visible-light absorption ability and enhanced PEC performance compared to g-CNS1 synthesized via the traditional one-step thermal polymerization method. Benefiting from its excellent PEC properties, the g-CNS3 exhibited high photocatalytic activity to removal MB with fast kinetics and served as the photoactive layer to construct a PEC immunosensor with high sensitivity and specificity for subgroup J avian leukosis virus detection. A linear range from 102.14 to 103.35 TCID50/mL and a detection limit of 102.08 TCID50/mL were obtained for the PEC immunoassay of the target virus. This work might provide a novel protocol for tailoring shaped 2D g-C3N4 nanosemiconductor with superior properties and shed light on its promising PEC applications.
关键词： Two-dimensional material,Photocurrent response,Graphitic carbon nitride,Photocatalysis,Photoelectrochemical immunosensor
更新于2025-09-23 15:23:52
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MIDAS projection
摘要： The visual appearance of an object can be disguised by projecting virtual shading as if overwriting the material. However, conventional projection-mapping methods depend on markers on a target or a model of the target shape, which limits the types of targets and the visual quality. In this paper, we focus on the fact that the shading of a virtual material in a virtual scene is mainly characterized by surface normals of the target, and we attempt to realize markerless and modelless projection mapping for material representation. In order to deal with various targets, including static, dynamic, rigid, soft, and fluid objects, without any interference with visible light, we measure surface normals in the infrared region in real time and project material shading with a novel high-speed texturing algorithm in screen space. Our system achieved 500-fps high-speed projection mapping of a uniform material and a tileable-textured material with millisecond-order latency, and it realized dynamic and flexible material representation for unknown objects. We also demonstrated advanced applications and showed the expressive shading performance of our technique.
关键词： material,photometric stereo,projection mapping,infrared
更新于2025-09-23 15:23:52
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One-drop Self-assembly and Size Control of Organic Nonlinear Optical Crystal DSNS Nanowires
摘要： In this study, we demonstrate a one-drop self-assembly method for fabricating nanowires (NWs) of organic second-order nonlinear optical (NLO) material, 4-N, N-dimethylamino-4'-N'-methyl- stilbazolium 2-naphthalenesulfonate (DSNS). By controlling the parameters of the self-assembly process, we successfully controlled the length of DSNS from a few micrometers to millimeters. The obtained NWs have very high surface quality with surface roughness <150 pm, which is highly beneficial for fabricating integrated optical devices. DSNS NW has the same triclinic crystal structure as that of bulk crystal and exhibits excellent second-order NLO and fluorescent properties, which could provide wide opportunities for on-chip optoelectronic devices and integrated photonic systems. Furthermore, the one-drop self-assembly method only requires reagents in microgram quantities, and thus this method is extremely environment-friendly.
关键词： one-drop self-assembly,organic nanowire,size control,nonlinear optical material
更新于2025-09-23 15:23:52
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Silicon-Based Embedded Trenches of Active Antennas for High-Responsivity Omnidirectional Photodetection at Telecommunication Wavelengths
摘要： Although the use of plasmonic nanostructures for photodetection below the band gap energy of the semiconductor has been intensively investigated recently, efficiencies of such hot electron-based devices have, unfortunately, remained low because of the inevitable energy loss of the hot electrons as they move and transfer in active antennas based on metallic nanostructures. In this work, we demonstrate the concept of high-refractive-index material-embedded trench-like (ETL) active antennas that could be used to achieve almost 100% absorbance within the ultrashallow region (approximately 10 nm) beneath the metal?semiconductor interface, which is a much smaller distance compared with the hot electrons’ mean free path in the noble metal layer. Taking advantage of these ETL-based active antennas, we obtained photoresponsivities under zero bias at wavelengths of 1310 and 1550 nm of 5854 and 693 nA mW?1, respectively—values higher than most those previously reported for active antenna-based silicon (Si) photodetectors that operate at optical telecommunication wavelengths. Furthermore, the ETL antenna strategy allowed us to preserve an omnidirectional and broadband photoresponse, with a superior degree of detection linearity of R2 = 0.98889 under the light of low power density (down to 11.1 μW cm?2). The photoresponses of the ETL antenna-based device varied by less than 10% upon changing the incident angle from normal incidence to 60°. Because these ETL-based devices provide high responsivity and omnidirectional detection over a broad bandwidth, they show promising potentials for use in hot electron-based optoelectronics for many applications (e.g., Si photonics, energy harvesting, photocatalysis, and sensing devices).
关键词： hot electron,embedded,plasmon,Schottky,high-refractive-index material
更新于2025-09-23 15:23:52
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Understanding Spatiotemporal Photocarrier Dynamics in Monolayer and Bulk MoTe <sub/>2</sub> for Optimized Optoelectronic Devices
摘要： Semiconducting molybdenum ditelluride has emerged as a promising transition-metal dichalcogenide with a number of novel properties. In particular, its bandgap in infrared range makes it an attractive candidate for ultrathin and high-performance infrared optoelectronic applications. Dynamical properties of photocarriers play a key role in determining performance of such devices. We report an experimental study on spatiotemporal dynamics of photocarriers in both monolayer and bulk MoTe2. Transient absorption measurement in reflection geometry revealed ultrafast thermalization and relaxation processes of photocarriers and lifetimes of about 60 and 80 ps in monolayer and bulk MoTe2, respectively. By spatially resolved transient absorption measurements on monolayer, we obtained an exciton diffusion coefficient of 20 ± 10 cm2 s?1, a mean free time of 200 fs, a mean free path of 20 nm, and a diffusion length of 350 nm. The corresponding values for the bulk sample are 40 ± 10 cm2 s?1, 400 fs, 40 nm, and 570 nm, respectively. These results provide fundamental information for understanding and optimizing performance of MoTe2-based optoelectronic devices.
关键词： two-dimensional material,exciton,transient absorption,molybdenum ditelluride,transition-metal dichalcogenide,diffusion,photocarrier dynamics
更新于2025-09-23 15:23:52