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oe1(光电查) - 科学论文

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?? 中文（中国） ▾

  • Thermal nanoimprint lithography based plasmonic nanogratings for refractive index sensing of polar solvents

    摘要： This work illustrates a facile approach for the design of flexible plasmonic sensors using gold nanograting. The fabrication of surface plasmon resonance (SPR) coupled refractive index (RI) sensor is proposed to sense the various known RIs of polar solvents. Thermal nanoimprint lithography (T-NIL) is used to transfer the nanograting of the processed digital versatile discs (DVDs) through polydimethylsiloxane (PDMS) stamp to thermoplastic polymer coated flexible polyethylene terephthalate (PET) substrate. The gold nanograting sample was obtained after the subsequent deposition of the gold thin film of thickness 60 nm on top of polymer nanograting. The surface plasmon resonance (SPR) modes excited on gold-encrusted polymer nanograting appeared as a dip in the reflectance spectra measured at normal incidence under white light in air and liquid medium. We use refractive index calibration polar solvents [methanol (1.331), water (1.333), acetone (1.359), ethanol (1.361) and isopropanol (1.382)] to determine the refractive index sensitivity of our gold nanograting arrays. This produces a bulk refractive index sensitivity of 535 ± 47 nm/RIU. The real-time kinetic response demonstrates the stability of the sensor with respect to the time and reusability of the sensing chip for multiple measurements. Thus, we envisaged that our proposed sensor can be a potential candidate for the development of highly sensitive plamonic device.

    关键词： Nanogratings,surface plasmon resonance (SPR),Thermal nanoimprint lithography (T-NIL),Plasmonic sensor,Polar solvents

    更新于2025-09-23 15:19:57

  • Dielectric and Ferroelectric Properties of P(VDF-TrFE) Films with Different Polar Solvents

    摘要： We investigated the structural, dielectric, and ferroelectric properties of poly(vinylidene fluoride-co-trifluoroethylene) [P(VDF-TrFE)] films that were grown using dimethylformamide (DMF) and tetrahydrofuran (THF) polar solvents. The DMF solvent has a large dipole moment with a long bond length and evaporates slowly while the THF solvent has a small dipole moment with a short bond length and evaporates rapidly. Because of these differences, a thin film with a rough surface occurs when using DMF while a thick film with a smooth surface is formed when using THF. Compared to DMF solvent, the ferroelectric polarization is not well saturated and the dielectric constant is quite low for the THF solvent, which is possibly due to the residual paraelectric defects in the P(VDF-TrFE) films. For both solvents, the polarization switching can be explained by using the Kolmogorov-Avrami-Ishibashi (KAI) model with similar switching times. Both solvents enable the P(VDF-TrFE) films to have good retention and fatigue resistance for ferroelectric polarization.

    关键词： Polar solvents,P(VDF-TrFE),Fatigue resistance,Ferroelectric switching,Retention

    更新于2025-09-19 17:15:36