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Quantumness in light harvesting is determined by vibrational dynamics
摘要: We demonstrate for the multi-level spin-boson (MLSB) Hamiltonian, typically used to describe biological light-harvesting, that the distinction between quantum and classical dynamics is determined entirely by the thermal environment. In particular, any MLSB model featuring classical interactions with a classical bath is exactly equivalent in its absorption and energy transfer dynamics to a classical model involving coupled harmonic oscillators. This result holds in the linear response regime for both pulsed and incoherent excitation. In the biological context, this finding highlights the centrality of vibrational dynamics in determining the 'quantumness' of photosynthetic light-harvesting, particularly in the creation of the photosynthetic energy funnel where excitation energy concentrates near the reaction center via a series of downhill energy transfer events. These findings support the idea that this energy funnel is exclusively quantum-mechanical in origin, although it need not rely on entanglement.
关键词: vibrational dynamics,energy transfer,photosynthesis,quantumness,light harvesting,spin-boson model
更新于2025-09-23 15:23:52
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Wehrl entropy based quantification of nonclassicality for single mode quantum optical states
摘要: Nonclassical states of a quantized light are described in terms of Glauber-Sudarshan P distribution which is not a genuine classical probability distribution. Despite several attempts, defining a uniform measure of nonclassicality (NC) for the single mode quantum states of light is yet an open task. In our previous work [Phys. Rev. A 95, 012330 (2017)] we have shown that the existing well-known measures fail to quantify the NC of single mode states that are generated under multiple NC-inducing operations. In this paper, we propose a new quantification of NC for the single mode quantum states as the difference between the total Wehrl entropy of the state and the maximum Wehrl entropy arising due to its classical characteristics. The classical reference state is chosen at the same randomness, given by the von-Neumann entropy, as the state itself. We further suggest operational interpretation of the proposed measure in terms of phase-space sampling entropy as well as potential to generate entanglement, in the case of pure states. We obtain analytic expressions of NC for pure states and Gaussian mixed states. We show that, along with the states generated under single NC-inducing operations, also for the broader class of states that are generated under multiple NC-inducing operations, our quantification enumerates the NC consistently. However, the evaluation of NC for the non-Gaussian mixed states is subject to extensive numerical computation that lies beyond the scope of the current work. We finally conclude with certain open questions.
关键词: Wehrl Entropy,Quantumness,Phase Space Distributions,Quantum Optics,Nonclassicality
更新于2025-09-23 15:21:01
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Quantum teleportation in terms of creation operators of photons
摘要: By using the formalism of photon creation operators, we present the simplest description of the effect of quantum teleportation and describe its closest classical analog.
关键词: creation operators,teleportation,state vectors,photons,classicality,quantumness
更新于2025-09-09 09:28:46