研究目的
Investigating the properties and excitation of Airy plasmon pulses using Multiphoton Photoemission Electron Microscopy (PEEM) in combination with a variable wavelength excitation from an optical parametric chirped pulse amplifier system (OPCPA).
研究成果
The excitation of stationary Airy plasmons is possible over a large bandwidth, but achieving ultrafast hotspots requires matching the spectral phase, which is difficult in dispersive systems. The study suggests that further improvements in the excitation scheme are needed for spatio-temporal hotspot creation.
研究不足
The creation of an ultrafast hotspot requires a matching of the spectral phase, which is challenging in strong dispersing systems. Further improvements of the excitation scheme are necessary to obtain spatio-temporal hotspots.
1:Experimental Design and Method Selection:
The study employs PEEM in combination with an OPCPA system to investigate Airy plasmon pulses emitted by an excitation grating. The method leverages the high intrinsic bandwidth of plasmonic excitation for ultrafast photonics.
2:Sample Selection and Data Sources:
The excitation grating consists of 11 rows of milled grooves separated by the distance d = λspp, where λspp = λ0/neff and neff = [εm/(εm + 1)]1/2 is the effective index of the SPP on the surface of a metal with permittivity εm.
3:List of Experimental Equipment and Materials:
PEEM, OPCPA system, excitation grating.
4:Experimental Procedures and Operational Workflow:
A normally incident light pulse excites the diffraction grating, emitting the Airy plasmon pulse, which alters the probability to emit a photoelectron, imaged by PEEM.
5:Data Analysis Methods:
The study includes rigorous finite-difference time domain simulations, a nonlinear electron yield model, and analytic calculations to determine the modal purity of the Airy plasmon excitation based on reciprocity.
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