摘要： As an inevitable optoelectronic material with unique properties, halide perovskites attracted increasing attention in recent years. Meanwhile, hybridization of nanostructured perovskites with one-dimensional (1D) or two-dimensional (2D) functional materials has exhibited unique applications in nanotechnology. In this communication, a highly conducting porous single-wall carbon nanotube (p-SWCNT) template decorated with phase-pure CsPbBr3 nanocrystals by simple solution-phase technique was demonstrated, and the ultra-flexible photodetector Au/p-SWCNT:CsPbBr3/Au showed high sensitivity even in highly bending state. Also, the mechanism of wetting CsPbBr3 along p-SWCNT and the detailed fabrication process for ultra-flexible photodetectors were highlighted. The direct contact (in-situ) on p-SWCNT by crystallization of perovskite precursor can enhance the charge transfer at their interface effectively. At applied bias of +5 V, the optimized photodetector Au/p-SWCNT:CsPbBr3/Au exhibits a maximum photoresponsivity of 41.0 AW-1 with a specific detectivity of 1.67×1012 Jones under an incident 232 μW/cm2 520 nm illumination. In addition, it exhibits excellent mechanical and electrical properties even under high strain (i.e. bending angle up to -17°) and recovers the original performance after repeated bending cycles upto 1000 times. Our experimental results showed that such a hybrid materials provide a promising method for rigid and flexible optoelectronic devices.