研究目的
To improve the power conversion efficiency (PCE) and stability of carbon-based perovskite solar cells (C-PSCs) through an innovative modular architecture design using graphene as the charge collector.
研究成果
The modular C-PSC configuration with graphene as the charge collector achieved a PCE of 18.65%, the highest reported for C-PSCs, with excellent stability and structural flexibility. This design opens new avenues for modular interconnection in advanced photovoltaic architectures.
研究不足
The study focuses on the modular design and graphene's role in C-PSCs but does not extensively explore other potential materials or configurations that might offer similar or better performance.
1:Experimental Design and Method Selection:
The study introduced a modular PSC design with a carbon back electrode, reduced in sheet resistance and thickness by covering it with another carbon-coated FTO glass under pressure.
2:Sample Selection and Data Sources:
Three commercial carbon sources (carbon black, graphite sheet, and graphene) were selected for comparison.
3:List of Experimental Equipment and Materials:
Carbon-coated FTO glass, SnO2 electron transfer layer (ETL), mixed-cation perovskite layer, spiro-OMeTAD HTL, and carbon layer.
4:Experimental Procedures and Operational Workflow:
Semi-cell A was fabricated at a low temperature by depositing layers sequentially, while charge collector B was obtained by depositing a carbon layer on an FTO/glass substrate. Modular C-PSCs were achieved by stacking charge collector B and semi-cell A under pressure.
5:Data Analysis Methods:
The performance was evaluated through power conversion efficiency (PCE), stability tests under humidity and heat, and structural flexibility tests.
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