研究目的
Investigating ultrafast nanoplasmonic dynamics via nonlinear photoemission from metallic nanostructures using a time-resolved normal-incidence photoemission electron microscope.
研究成果
The study successfully demonstrated the capability of visualizing few-femtosecond nanoplasmonic dynamics with high spatial and temporal resolution, paving the way for future research in ultrafast nanoplasmonic field visualization.
研究不足
The study is limited by the technical constraints of achieving ultimate spatiotemporal resolution and the potential for space charge effects to influence the results.
1:Experimental Design and Method Selection:
Utilized a time-resolved normal-incidence photoemission electron microscope with an imaging time-of-flight detector and a phase-stabilized interferometer.
2:Sample Selection and Data Sources:
Studied a monolayer of self-assembled gold nanospheres with ~40 nm diameter and ~2 nm interparticle distance.
3:List of Experimental Equipment and Materials:
Included a Ti:sapphire oscillator, Mach-Zehnder type interferometer, and a normal-incidence photoemission electron microscope.
4:Experimental Procedures and Operational Workflow:
Conducted delay scans over an optical delay range with specific step sizes and integration times.
5:Data Analysis Methods:
Analyzed data using fast Fourier transformation and energy filtering techniques.
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