研究目的
To explore the epitaxial growth of multi-layer InGaAs/GaAs quantum dot heterostructures on Ge substrates and compare the optical and structural properties with the QDs grown on GaAs substrate, aiming to overcome the impediment to Si-photonics through monolithic integration of optoelectronic device structures.
研究成果
The incorporation of SLB layers in the growth of InGaAs/GaAs quantum dot heterostructures on Ge substrates significantly enhances optical and structural properties by minimizing defects and dislocations. Ex-situ H ion-implantation further improves optical characteristics, making the heterostructures comparable to those grown on GaAs substrates. This approach is promising for silicon photonics applications.
研究不足
The study acknowledges the challenges of direct growth of III-V nanostructures on Si due to large lattice mismatch and the generation of anti-phase domains (APDs) and dislocations at the polar (GaAs) and non-polar (Si) semiconductor interface, which can degrade device efficiency.
1:Experimental Design and Method Selection:
The study involved the epitaxial growth of InGaAs/GaAs quantum dot heterostructures on Ge substrates using molecular beam epitaxy (MBE) and compared their properties with those grown on GaAs substrates. Optical properties were investigated using photoluminescence (PL) and time-resolved photoluminescence (TRPL), while structural properties were examined via cross-sectional transmission electron microscopy (XTEM).
2:Sample Selection and Data Sources:
Three samples were grown: two on Ge substrates (one with and one without a super-lattice buffer (SLB) layer) and one on a GaAs substrate as a reference.
3:List of Experimental Equipment and Materials:
Solid source molecular beam epitaxy (Riber: Epineat III-V) system, valved Arsenic-cracker source, helium-cryostat for PL measurements, green (532 nm) laser, Liquid Nitrogen (LN2) cooled InGaAs detector array, picosecond pulsed 510-nm Pico-Quant laser for TRPL measurements, Micromath scientist software for data analysis, cross-sectional transmission electron microscopy (XTEM) for structural characterization.
4:Experimental Procedures and Operational Workflow:
The growth process included the deposition of MEE GaAs layer, GaAs buffer layer, SLB layer (for one sample), and InGaAs QD layers. Optical and structural characterizations were performed post-growth.
5:Data Analysis Methods:
PL and TRPL data were analyzed to assess optical properties, while XTEM images were used to evaluate structural properties. Activation energies were calculated using the Arrhenius equation.
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Molecular beam epitaxy system
Epineat III-V
Riber
Used for the epitaxial growth of InGaAs/GaAs quantum dot heterostructures on Ge substrates.
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Arsenic-cracker source
Embedded in the MBE system for the growth process.
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Helium-cryostat
Used for photoluminescence (PL) measurements to observe the optical behavior of each sample.
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Green laser
Used as the excitation source for PL measurements.
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InGaAs detector array
Used to detect the emission from the sample during PL measurements.
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Picosecond pulsed laser
510-nm Pico-Quant
Used as the excitation source for time-resolved photoluminescence (TRPL) measurements.
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Micromath scientist software
Used for analyzing photoluminescence decays.
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Cross-sectional transmission electron microscopy (XTEM)
Used to observe the morphology of the QDs.
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Horiba integrated triple spectrometer
T64000
Used for room temperature non-resonant Raman scattering in backscattering geometry.
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Ar + laser
Used for excitation in Raman scattering measurements.
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Si charge-coupled detector (CCD) camera
Used to detect Raman signals.
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