研究目的
Investigating the low-threshold stimulated emission in perovskite quantum dots induced by surface plasmon polaritons at room temperature.
研究成果
The work demonstrates low-threshold lasing of perovskite QDs in the single-exciton regime, facilitated by plasmon resonance energy transfer. This approach may provide a new concept for the design of low-threshold lasing of colloids in the single-exciton regime and the miniaturization of coherent light sources.
研究不足
The study is limited by the low loading level of the perovskite QDs in the mesoporous nanocomposite structure system compared to absolute perovskite QDs samples.
1:Experimental Design and Method Selection:
The study employs a metal surface plasmon resonance energy-transfer effect to achieve optical gain in the single-exciton regime.
2:Sample Selection and Data Sources:
Colloidal perovskite quantum dots loaded in a gold–porous silicon core–shell nanocomposite structure were used.
3:List of Experimental Equipment and Materials:
UV/vis absorption spectroscopy, femtosecond transient-absorption spectral measurements, and optical fiber spectrometer were used.
4:Experimental Procedures and Operational Workflow:
The optical properties were analyzed by UV/vis absorption spectroscopy. Spectra were recorded for the colloidal solution of CsPbBr3 QDs loaded in the porous silicon shell with and without an Au core.
5:Data Analysis Methods:
The kinetic signals were analyzed by a fitting procedure using Igor Pro software.
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