研究目的
Investigating the transient changes of the optical properties, specifically re?ectivity, of gold under intense femtosecond laser irradiation, and understanding the mechanisms behind these changes.
研究成果
The study provides a comprehensive understanding of the transient changes of collision frequencies and their dependence on temperature for the description of energy absorption in laser-excited gold. The approach represents a powerful tool for describing the most general case of laser self-re?ectivity and its precise absorbed energy at a certain time and location for elevated electronic temperatures.
研究不足
The study does not account for effects like two photon absorption, fluorescence, or an onset of a plasma state at very high peak fluences. It also neglects effects of a non-Fermi distribution of the excited electrons.
1:Experimental Design and Method Selection:
The study involves measurements of the re?ectivity of laser-excited gold in the infrared and ultraviolet ranges, using a theoretical scheme based on the two-temperature model with the electronic temperature as the key parameter.
2:Sample Selection and Data Sources:
Polycrystalline gold films deposited by evaporation technique on a polished glass surface with a 50 nm chromium layer for enhanced adhesion.
3:List of Experimental Equipment and Materials:
Ti:Sapphire regenerative amplifier system for IR experiments, frequency tripled and amplified in a KrF excimer module for UV experiments, various energy detectors, and a home-made UV-FROG for pulse length determination.
4:Experimental Procedures and Operational Workflow:
Laser pulses are reflected under nearly normal incidence by a gold target, and the incident and reflected energy of the pulse are measured.
5:Data Analysis Methods:
The data is analyzed using a theoretical scheme based on all-electron calculations of the interband contribution to the re?ectivity and a careful determination of the intraband, Drude-like terms.
独家科研数据包,助您复现前沿成果,加速创新突破
获取完整内容-
Ophir PE9-ES-C
PE9-ES-C
Ophir
Energy detector used in the experiment.
-
Ophir PD10-C
PD10-C
Ophir
Energy detector used in the experiment.
-
Polytec RjP-735
RjP-735
Polytec
Energy detector used in the experiment.
-
Ophir PE10BF-C
PE10BF-C
Ophir
Energy detector used in the experiment.
-
Ti:Sapphire regenerative amplifier system
Used for IR experiments to generate laser pulses.
-
KrF excimer module
Used for frequency tripling and amplifying Ti:Sapphire pulses for UV experiments.
-
UV-FROG
Home-made device used for pulse length determination.
-
Positive Light single shot autocorrelator
Positive Light
Used for determining the pulse length in the IR range.
-
登录查看剩余6件设备及参数对照表
查看全部