研究目的
Developing white light-emitting diodes (WLEDs) for lightings with high color rendering index (CRI), low correlated color temperature (CCT), and displays with wide color gamut using inorganic perovskite quantum dots (QDs) such as CsPbX3 (X = Cl, Br, I).
研究成果
The study successfully synthesized green and red perovskite QD powders such as Cs4PbBr6 and Cs4Pb(Br0.4I0.6)6 with improved quantum efficiency and long lifetime. These QD powders were applied to high-quality WLEDs for lightings and displays, showing outstanding potential applications.
研究不足
The study mentions the poor air stability and severe decline of quantum efficiency in CsPbBr3 QDs in the form of powders or films. The use of highly dangerous and corrosive hydrofluoric acid (HF) during preparation of fluoride phosphors is also a limitation.
1:Experimental Design and Method Selection:
The study proposed a new idea of developing 0-D green–red perovskite QDs powders such as Cs4PbBr6 and Cs4Pb(Br
2:4I6)6 with improved quantum efficiency and long lifetime by silica-coated method and crystal phase transition in low-temperature synthesis. Sample Selection and Data Sources:
The samples used were green and red perovskite QD powders synthesized at 140°C.
3:List of Experimental Equipment and Materials:
The materials included Cs4PbBr6 and Cs4Pb(Br
4:4I6)6 QD powders, commercial YAG phosphors, and blue chips. Experimental Procedures and Operational Workflow:
The QD powders were combined with blue chips to fabricate WLEDs for displays and lightings. The performance of these devices was measured under different driving currents.
5:Data Analysis Methods:
The optical properties, crystal structure, surface morphology, and air stability of the QD powders were studied. The performance of the WLEDs was evaluated based on CRI, CCT, and luminous efficiency.
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