研究目的
Investigating the interaction between a nanosecond laser produced plasma and a unipolar high voltage discharge to enhance the laser-induced breakdown spectroscopy (LIBS) emission.
研究成果
The study concluded that the interaction between a laser-produced plasma and a high voltage discharge significantly enhances LIBS emission, primarily through an increase in plasma ionization degree rather than mass removal. The enhancement is more pronounced at lower laser fluences and results in longer plasma duration and greater enhancement of ionic species compared to neutrals. The findings suggest that further optimization of the discharge timing could enhance emission even more.
研究不足
The study's limitations include the technical constraints of the experimental setup, such as the fixed timing of the electrical discharge and the spatial resolution of the fast photography. Potential areas for optimization include adjusting the delay between the laser pulse and the electrical discharge for higher fluences.
1:Experimental Design and Method Selection:
The study employed time-resolved spectroscopy, fast photography with narrow band interference filters, and profilometry to analyze the interaction between a laser-produced plasma and a high voltage discharge. The laser ablation fluence was varied in the 60–1000 J/cm2 range.
2:Sample Selection and Data Sources:
An aluminum target was used, with spectra obtained from a spot 1 mm above the target.
3:List of Experimental Equipment and Materials:
A Nd: YAG laser (Continuum, Surelite III), a 50 cm Czerny-turner spectrograph (Acton Research, Spectra Pro 2500i), an intensi?ed CCD camera (Princeton Instruments, PiMAX 1024 × 1024), and a DC high voltage power supply (Bertan, 205B) were used.
4:Experimental Procedures and Operational Workflow:
The high voltage discharge was triggered by an ablation plasma on the aluminum target at time 700 ns. The emitted light was collected and analyzed for time-integrated and time-resolved measurements.
5:Data Analysis Methods:
The emission lines were fitted to a Lorentzian function to obtain line intensities and widths. Plasma temperature and electron density were calculated using the Saha-Boltzmann method and Stark broadening, respectively.
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