研究目的
Investigating the tropospheric NO2, SO2, and HCHO over the East China Sea using ship-based MAX-DOAS observations and comparing with OMI and OMPS satellites data.
研究成果
The study provided further understanding of the main air pollutants in the marine boundary layer of the ECS area and highlighted the strong impacts of shipping emissions on the air quality, which need to be regulated urgently in the coming future, especially for the YRD region where the world top 2 ports are located.
研究不足
The study is limited by the spatial and temporal coverage of the ship-based measurements and the potential impacts of local ship emissions on the observed trace gas concentrations.
1:Experimental Design and Method Selection:
Ship-based MAX-DOAS measurements were performed in the Eastern China Sea (ECS) area in June
2:The tropospheric Slant Column Densities (SCDs) of NO2, SO2, and HCHO were retrieved from the measured spectra by the DOAS technique. Sample Selection and Data Sources:
20 The cruise ship mainly navigated at the sea area surround Yangtze River Delta (YRD) region.
3:List of Experimental Equipment and Materials:
An integrated and fully automated MAX-DOAS instrument was used, consisting of an ultraviolet spectrometer, a one-dimensional CCD detector, and a stepper motor driven telescope.
4:Experimental Procedures and Operational Workflow:
The telescope was scanning in the sequence of elevation angles of 3o, 5o, 7o, 10o, 15o, 30o, and 90o. The duration of an individual spectrum measurement was about 30 s.
5:0o. The duration of an individual spectrum measurement was about 30 s. Data Analysis Methods:
5. Data Analysis Methods: The measured scattered sun-light spectra are analyzed using the QDOAS spectral fitting software suite.
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AvaSpec-ULS2048L-USB2
AvaSpec-ULS2048L-USB2
Avantes
Ultraviolet spectrometer covering the spectral range of 300-460 nm with a spectral resolution of 0.6 nm.
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Sony ILX511
ILX511
Sony
One-dimensional CCD detector with 2048 individual pixels.
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QDOAS
QDOAS
BIRA-IASB
Spectral fitting software suite for analyzing measured scattered sun-light spectra.
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OMI
Ozone Monitoring Instrument
NASA
Monitoring ozone, NO2, and other minor trace gases distribution with high spatial resolution.
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OMPS
Ozone Mapping and Pro?ler Suite
NASA
Monitoring ozone and other trace gases with high spatial resolution.
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