研究目的
To analyze the magnetic field generated by a continuous current in metallic microwires on a diamond substrate using NV magnetometry and resolve an apparent anomaly in the field measurements.
研究成果
The study identifies an anomaly in magnetic field measurements from currents in metallic wires on diamond, where the field components violate classical electrodynamics laws under the assumption of current confinement to the wire. By allowing current sources above and below the NV layer, the data are fully explained, indicating significant current flow in the diamond with lateral spread. No actual electrical conduction occurs, ruling out conventional effects. The anomaly is robust across samples and conditions, suggesting it may impact NV magnetometry applications in charge transport studies, and further investigation is needed to understand the underlying physics.
研究不足
The experiments are limited to room temperature and specific diamond samples with NV layers at shallow depths. The spatial resolution is constrained by the optical diffraction limit (~500 nm). Systematic errors in magnetic field measurements (up to 2 μT) and truncation artifacts in current density reconstruction affect accuracy. The apparent current delocalization into the diamond lacks a clear physical explanation and may be influenced by laser intensity and NV layer properties.
1:Experimental Design and Method Selection:
The experiment uses NV centers in diamond as vector magnetometers to image the stray magnetic field from dc currents in metallic wires. Pulsed optically detected magnetic resonance (ODMR) spectroscopy is employed to measure Zeeman shifts in NV spins, with a custom-built wide-field fluorescence microscope.
2:Sample Selection and Data Sources:
Single-crystal diamond plates implanted with nitrogen ions at various energies and fluences to form NV layers at depths from 8 nm to 28 nm. Metallic wires (Ti/Au or Cr/Au) are fabricated on the diamond by photolithography and electron-beam evaporation.
3:List of Experimental Equipment and Materials:
Diamond substrates, nitrogen ion implanter, photolithography setup, electron-beam evaporator, green laser (532 nm), microwave antenna, current source, sCMOS camera, pulse pattern generator, and various materials like Ti, Cr, Au, Al2O3, and graphene.
4:Experimental Procedures and Operational Workflow:
Fabricate NV-diamond samples and metallic wires. Mount the device on a coverslip with electrical connections. Use the microscope to perform ODMR measurements with and without applied current. Record PL images and ODMR spectra, fit the spectra to extract magnetic field components, and subtract background fields to isolate current-induced fields.
5:Data Analysis Methods:
Fit ODMR spectra with Lorentzian functions to determine resonance frequencies. Use the NV spin Hamiltonian to compute magnetic field components. Apply Biot-Savart law, Ampère's law, and Gauss's law for magnetism. Reconstruct current densities using Fourier transforms and inversion techniques.
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Camera
Neo
Andor
Imaging NV photoluminescence
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Signal Generator
SMBV100A
Rohde & Schwarz
Generating microwave signals for ODMR
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Source-Meter Unit
SMU 2450
Keithley
Applying and measuring dc current
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Acousto-Optic Modulator
MQ180-A0,25-VIS
AA Opto-Electronic
Gating the laser beam
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Laser
Opus
Laser Quantum
Optical excitation of NV centers
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Amplifier
60S1G4A
Amplifier Research
Amplifying microwave signals
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Pulse Pattern Generator
PulseBlasterESR-PRO 500 MHz
SpinCore
Gating laser and microwave pulses
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Objective Lens
CFI S Fluor 40x
Nikon
Focusing laser light and collecting PL
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