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Planar plasmonic nanocavity for efficient enhancement of photoluminescence of molecular emitters
摘要： Effects of plasmonic gap mode formation due to coupling between metal nanoparticles and thin metal film separated by thin dielectric luminescent film-spacer (gap) have been studied by means of light extinction and photoluminescence in three-layer planar Au NPs monolayer/shellac-dye film/Au film nanostructure with spacer thickness varied in the range 8–47 nm. The 3-fold enhancement of light extinction and 90 nm red shift of the plasmon mode have been observed in extinction spectra. The 37-fold enhancement of dye photoluminescence and the significant (48 nm) red shift of dye photoluminescence band have been observed for Au NPs monolayer/shellac-dye film/Au film nanostructure in comparison with bare shellac-dye film for the spacer thickness of 8 nm. The decrease of the spacer thickness causes the increase of the enhancement factor of dye photoluminescence indicating the strengthening of the gap mode field. FDTD calculations of the dependence of the intensity of the field of gap mode on the gap thickness have demonstrated good quantitative agreement with experimental data that proves the key role of gap mode in the enhancement of the electromagnetic field in planar metal NPs monolayer/dielectric film/metal film plasmonic nanocavity nanostructures. The variation of the gap thickness provides the possibility to tune controllably the spectral position and enhancement factor of the light emission from the molecular emitters located in the gap that can be used in the novel nanophotonics devices and for highly sensitive detection of the single molecules.
关键词： Near field coupling,Gap thickness dependence,Molecular emitters,Gap mode,Plasmonic nanocavity,Photoluminescence enhancement
更新于2025-11-19 16:46:39
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Rabi Oscillation Study of Strong Coupling in a Plasmonic Nanocavity
摘要： Strong interaction between emitters and plasmonic nanocavity has various applications in quantum fields at room temperature. As Rabi oscillation gives the direct proof to the energy exchange in strong coupling, it is more intuitive and necessary to analyze the interaction in time domain. In this paper, we give the Rabi oscillation in a high-dissipation plasmonic nanocavity by using full-quantum method and draw a new strong coupling criterion about mode volume which provides a significant guidance in plasmonic nanocavitys nanofabrication. Moreover, we reveal the relation between Rabi oscillation and Rabi splitting, which is beneficial for exploring emitter-plasmon hybrid systems time-domain property through frequency-domain response. An emitter-hexagon hybrid system with ultrasmall mode volume is designed to verify our theory. The numerical simulation shows good agreements with our theoretical results. Our work has applications in quantum information and quantum computing in the future.
关键词： plasmonic nanocavity,quantum information,Rabi oscillation,quantum computing,strong coupling
更新于2025-09-23 15:21:01
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Strong Exciton-Plasmon Coupling and Hybridization of Organic-Inorganic Exciton-Polaritons in Plasmonic Nanocavity <sup>*</sup>
摘要： We investigate strong exciton-plasmon coupling and plasmon-mediated hybridization between the Frenkel (F) and Wannier–Mott (WM) excitons of an organic-inorganic hybrid system consisting of a silver ring separated from a monolayer WS2 by J-aggregates. The extinction spectra of the hybrid system calculated by employing the coupled oscillator model are consistent with the results simulated by the finite-difference time-domain method. The calculation results show that strong couplings among F excitons, WM excitons, and localized surface plasmon resonances (LSPRs) lead to the appearance of three plexciton branches in the extinction spectra. The weighting efficiencies of the F exciton, WM exciton and LSPR modes in three plexciton branches are used to analyze the exciton-polaritons in the system. Furthermore, the strong coupling between two different excitons and LSPRs is manipulated by tuning F or WM exciton resonances.
关键词： coupled oscillator model,finite-difference time-domain method,localized surface plasmon resonances,plasmonic nanocavity,exciton-plasmon coupling,Frenkel excitons,organic-inorganic hybrid system,Wannier–Mott excitons
更新于2025-09-23 15:21:01
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Metallic Carbon Nanotube Nanocavities as Ultra-compact and Low-loss Fabry-Perot Plasmonic Resonators
摘要： Plasmonic resonators enable deep subwavelength manipulation of light matter interactions and have been intensively studied both in fundamental physics as well as for potential technological applications. While various metallic nanostructures have been proposed as plasmonic resonators, their performances are rather limited at mid- and far-infrared wavelengths. Recently, highly-confined and low-loss Luttinger liquid plasmons in metallic single walled carbon nanotubes (SWNTs) have been observed at infrared wavelengths. Here, we tailor metallic SWNTs into ultraclean nanocavities by advanced scanning probe lithography and investigate plasmon modes in these individual nanocavities by infrared nano-imaging. The dependence of mode evolutions on cavity length and excitation wavelength can be captured by a Fabry-Perot resonator model of a plasmon nanowaveguide terminated by highly reflective ends. Plasmonic resonators based on SWNT nanocavities approach the ultimate plasmon confinement limit and open the door to the strong light-matter coupling regime, which may enable various nanophotonic applications.
关键词： Plasmonic nanocavity,Carbon nanotubes,Nanophotonics,Infrared nano-imaging
更新于2025-09-19 17:13:59
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[IEEE 2019 44th International Conference on Infrared, Millimeter, and Terahertz Waves (IRMMW-THz) - Paris, France (2019.9.1-2019.9.6)] 2019 44th International Conference on Infrared, Millimeter, and Terahertz Waves (IRMMW-THz) - Plasmonic Nanocavities for High-Responsivity and Broadband Terahertz Detection
摘要： We present a high-responsivity and broadband photoconductive terahertz detector based on a plasmonic nanocavity, which enables high quantum efficiency and ultrafast operation without using short-carrier-lifetime substrates. We experimentally demonstrate that a time-domain spectroscopy setup employing the presented detector can offer 102 dB dynamic range over 0.1-4.5 THz.
关键词： high-responsivity,photoconductive detector,plasmonic nanocavity,broadband,terahertz
更新于2025-09-12 10:27:22