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Two dimensional temperature measurement characteristics in pulverized coal combustion field by computed tomography-tunable diode laser absorption spectroscopy
摘要： Two dimensional temperature and concentration distributions are important parameters for pulverized coal combustion used for power plant to understand the combustion field and develop the high efficient combustion technologies. However, it is difficult to measure two dimensional temperature and concentration in pulverized coal combustion field using conventional measurement technologies because pulverized coal combustion produces lots of dust and strong emission from its flame. This paper focused on the application of two dimensional temperature measurement method based on the combination of computed tomography and tunable diode laser absorption spectroscopy using absorption spectra of water vapor at 1388nm and 1343nm for each laser scanning using direct absorption spectroscopy, which show the better characteristics of spatial-temporal resolution, fast response, high sensitivity, self-calibration and optical accessibility. Accuracy of temperature measurement using tunable diode laser absorption spectroscopy was improved by applying the corrected spectroscopic database. Computed tomography reconstruction accuracy of 16 laser-paths configuration was evaluated using sum of squared difference (0.001) and zero-mean normalized cross-correlation (over 0.991), which presented the consistent temperature between assumed and reconstructed distributions. This developed computed tomography-tunable diode laser absorption spectroscopy was successfully applied to pulverized coal flame for two dimensional temperature measurement with 1 ms temporal resolution for time-series two dimensional temperature measurement in the range of 300K-2500K. The rationality was demonstrated by comparison of pulverized coal flame and Methane-Air flame temperature distributions due to the main heat release produced by methane fuel. Its applicability to pulverized coal combustion field will be benefit for optimal operation control and combustion efficiency improvement by combustion organization or new design of combustion system.
关键词： Power plant,Pulverized coal combustion,Computed tomography (CT),Tunable diode laser absorption spectroscopy (TDLAS),Two dimensional temperature measurement
更新于2025-09-23 15:21:01
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EXPRESS: Influence of Line Pair Selection on Flame Tomography Using Infrared Absorption Spectroscopy
摘要： We report the influence of absorption line selection on the tomographic results for high-temperature flames by numerical and experimental methods. Different combinations of infrared H2O absorption transitions are utilized with the Tikhonov-regularized Abel inversion to reconstruct the radial distribution of temperature and H2O concentration in a flat flame. It is shown that besides using the mathematical algorithm such as regularization, selecting a line pair with a large ΔE″ (> 1390 cm–1) also reduces the reconstruction uncertainty at 300–2000 K. In this study, a proper selection of absorption line pairs reduces the reconstruction uncertainty by 25% at the same level of noise. The line pair of H2O transitions at 4029.524 cm–1 and 4030.729 cm–1 is recommended for the tomography of high-temperature flames at 1000–3000 K, whereas the line pair of 7185.597 cm–1 and 7444.352 cm–1 can be used at 300–1000 K.
关键词： tunable diode laser absorption spectroscopy,TDLAS,Tomography,high-temperature flame,line selection
更新于2025-09-23 15:21:01
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Experimental observation of the vibration-rotation radiation curves of <sup>12</sup> C <sup>16</sup> O <sub/>2</sub> and <sup>13</sup> C <sup>16</sup> O <sub/>2</sub> absorption constants ranging from 4860 to 4880 sm <sup>a??1</sup> by the tunable diode laser absorption spectroscopy method
摘要： We report the experimental observation of the absorption constant values of 12C16O2 and 13C16O2 using the tunable diode laser absorption spectroscopy method ranging from 4860 to 4880 sm?1 within the pressure limits of 8–240 mbar for the absorption curves (lines) R(18), R(20), R(22), R(24), R(26), R(28), R(30), R(32), R(34) and R(36) of the 20013–00001 molecule 12C16O2 vibration band, and within the pressure limits of 0.06–1.7 mbar for the absorption curves P(10), P(12), P(14), P(16), P(18), P(20) and P(22) of the 20012–00001 molecule 13C16O2 vibration band. In the work, as a mixture under analysis, a mixture of the isotopes 13C16O2 and 12C16O2 at the ratio of 1:140 was used. The results have been compared with the data of the HITRAN spectroscopic database.
关键词： tunable diode laser absorption spectroscopy,carbon dioxide,absorption coefficients
更新于2025-09-23 15:19:57
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Gas distribution mapping for indoor environments based on laser absorption spectroscopy: Development of an improved tomographic algorithm
摘要： Gas distribution mapping (GDM) is an important technology for the study of indoor environment, which can be used to evaluate the efficiency of environmental control system and identify pollutant sources. Most recent studies have implemented GDM through contact sensors or a sensor network, which is difficult to calibrate all the sensors and cover the whole space. In this study, we introduced the non-contact tunable diode laser absorption spectroscopy (TDLAS) technology for GDM in the indoor environment. An improved tomographic algorithm, namely Least Square with Tikhonov Regularization (LSTR), was proposed and compared with two available tomographic algorithms using four validated computational fluid dynamics (CFD) simulations. We also analyzed the effects of the laser emitter placements and optical path densities on the concentration field reconstruction quantitatively. The results showed that the LSTR method could reduce the average relative root mean square error (RRMSE) of tomography by 52%, and the laser emitter at the long edge middle (LEM) can achieve better tomographic performance. The degree of the concentration dispersion from the source would mainly impact the tomographic results: when the sector dispersion (SD) value of concentration distribution was about 2.3 times larger, the average RRMSE value would be decreased by about 40%. The intersection matrix with a higher path density achieved a more accurately reconstructed map due to its lower condition number. In addition, the optical path density was suggested to twice the number of grid cells considering the trade-off between scanning time and accuracy.
关键词： Non-contact sensing,Tunable diode laser absorption spectroscopy (TDLAS),Concentration measurement,Indoor air,Air pollution
更新于2025-09-23 15:19:57
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Pulverized coal combustion application of laser-based temperature sensing system using computed tomography a?? Tunable diode laser absorption spectroscopy (CT-TDLAS)
摘要： The investigation of combustion phenomena in pulverized coal flames is significant for combustion optimization related to energy conservation and emission reduction. Real-time two dimensional (2D) temperature and concentration distributions play an important role for combustion analysis. The non-contact and fast response 2D temperature and concentration distribution measurement method was developed in this study. The method is based on a combination of computed tomography (CT) and tunable diode laser absorption spectroscopy (TDLAS). The accuracy evaluation of developed 32-path CT-TDLAS demonstrated its feasibility of 2D temperature measurement. 32-path CT-TDLAS was applied to CH4 and 5 kg/h coal combustion fields for 2D temperature measurement. The time-series 2D temperature distribution in coal combustion furnace was measured using 32-path CT-TDLAS measurement cell with kHz time resolution. The transient temperature field of combustion flame directly reflects the combustion mode and combustion stability. The measurement results demonstrate its applicability of CT-TDLAS to various types of combustor, especially the combustion fields with coal and ash particles. CT-TDLAS method with kHz response time enables the real-time 2D temperature measurement to be applicable for combustion analysis.
关键词： 2D temperature measurement,Computed tomography (CT),Tunable diode laser absorption spectroscopy (TDLAS),Time-series distribution,Coal combustion
更新于2025-09-23 15:19:57
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Spectral Line Shape Analysis Using Hartmann-Tran Profile for Tunable Diode Laser Absorption Spectroscopy of Water Vapor at 1.39a????m
摘要： In this study, spectral line shape analysis was conducted for water vapor absorption at 1.39 μm with a Hartmann-Tran pro?le (HTP), which is capable of being ef?ciently and accurately reduced to (speed dependent) Voigt and (speed dependent) Rautian pro?les. The near-IR absorption lines of water vapor were measured using tunable diode laser absorption spectroscopy (TDLAS). The spectrum ?tting code was home-written based on the Trust region re?ective algorithm and the HTP. Voigt pro?le (VP), Rautian pro?le (RP), speed-dependent VP (SDVP), and speed-dependent Rautian pro?le (SDRP), which were reduced from the HTP, were used as model functions to test the validity of the near-IR absorption lines of water vapor in terms of line shape pro?le. With the SDVP, the standard deviation of the ?tting residuals was at a 10?3 level relative to the most intense peak height in a range of 1.39 μm at 2.5 Torr and room temperature, while the global standard deviation was less than 0.5 × 10?3, thus showing the best result among them. This suggests the need to consider the speed-dependent collision width in the self-broadening of water vapor.
关键词： Tunable diode laser absorption spectroscopy,Hartmann-Tran pro?le,Spectral lineshape analysis,Water vapor
更新于2025-09-23 15:19:57
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Near-infrared tunable diode laser absorption spectroscopy-based determination of carbon dioxide in human exhaled breath
摘要： A spectroscopic detection system for the accurate monitoring of carbon dioxide (CO2) in exhaled breath was realized by tunable diode laser absorption spectroscopy (TDLAS) in conjunction with a vertical-cavity surface-emitting laser (VCSEL) and a multipass cell with an effective optical path-length of 20 m. The VCSEL diode emitting light with an output power of 0.8 mW, covered the strong absorption line of CO2 at 6330.82 cm?1 by drive-current tuning. The minimum detectable concentration of 0.769% for CO2 detection was obtained, and a measurement precision of approximately 100 ppm was achieved with an integration time of 168 s. Real-time online measurements were carried out for the detection of CO2 expirograms from healthy subjects, different concentrations were obtained in dead space and alveolar gas. The exhaled CO2 increased significantly with the increasing physical activity, reaches its maximal value at the beginning of respiratory compensation and then decreased slightly until maximal exercise. The developed measurement system has a great potential to be applied in practice for the detection of pulmonary diseases associated with CO2 retention.
关键词： CO2,human health monitoring,Tunable diode laser absorption spectroscopy,carbon dioxide,VCSEL,exhaled breath,TDLAS,vertical-cavity surface-emitting laser
更新于2025-09-16 10:30:52
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EXPRESS: Two-Dimensional Temperature Measurement in a High Temperature and Pressure Combustor Using Computed Tomography Tunable Diode Laser Absorption Spectroscopy (CT-TDLAS) with a Wide-Scanning Laser at 1335–1375 nm
摘要： Tunable diode laser absorption spectroscopy (TDLAS) technology is a developing method for temperature and species concentration measurements with the features of non-contact, high precision, high sensitivity, etc. The difficulty of two-dimensional (2D) temperature measurement in actual combustors has not yet been solved because of pressure broadening of absorption spectra, optical accessibility, etc. In this study, the combination of computed tomography (CT) and TDLAS with a wide scanning laser at 1335–1375 nm has been applied to a combustor for 2D temperature measurement in high temperature of 300–2000 K and high pressure of 0.1–2.5 MPa condition. An external cavity type laser diode with wide wavelength range scanning at 1335–1375 nm was used to evaluate the broadened H2O absorption spectra due to the high temperature and high pressure effect. The spectroscopic database in high temperature of 300–2000 K and high pressure of 0.1–5.0 MPa condition has been revised to improve the accuracy for temperature quantitative analysis. CT reconstruction accuracy was also evaluated in different cases, which presented the consistent temperature distribution between CT reconstruction and assumed distributions. The spatial and temporal distributions of temperature in the high temperature and high pressure combustor were measured successfully by CT-TDLAS using the revised spectroscopic database.
关键词： high temperature and high pressure field,TDLAS,computed tomography,2D,Two-dimensional temperature measurement,combustion,CT,tunable diode laser absorption spectroscopy
更新于2025-09-12 10:27:22
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Influence of Light Coupling Configuration and Alignment on the Stability of HWG-Based Gas Sensor System for Real-Time Detection of Exhaled Carbon Dioxide
摘要： A mid-infrared tunable diode laser absorption spectroscopy (TDLAS) gas sensor based on hollow waveguide (HWG) gas cell for real-time exhaled carbon dioxide (eCO2) detection is reported. A 2.73 μm distributed feedback (DFB) laser was used to target a strong CO2 absorption line, and wavelength modulation spectroscopy (WMS) with the second harmonic (WMS-2 f ) was used to retrieve the CO2 concentration with high sensitivity. The influence of different parameters, including coupling configuration of HWG, laser-to-HWG and HWG-to-detector coupling alignment on the stability of the HWG sensor is systematically studied. The HWG eCO2 sensor showed a fast response time of 2.7s, detection limit of 17 ppmv, and measurement precision of 20.9 ppmv with a 0.54 s temporal resolution. The eCO2 concentrations changed in breath cycles were measured in real time. The Allan variance indicated that the detection limit can reach 1.7 ppmv, corresponding to a detection sensitivity of 1.3×10?8 cm?1 Hz?1/2, as the integration time increases to 26 s. This work demonstrates the performance characteristics and merits of HWG eCO2 sensor for exhaled breath analysis and potential detection for other exhaled gases.
关键词： hollow waveguide,distributed feedback laser,carbon dioxide,Tunable diode laser absorption spectroscopy
更新于2025-09-11 14:15:04
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Simultaneous two cross-sectional measurements of NH<sub>3</sub> concentration in bent pipe flow using CT-tunable diode laser absorption spectroscopy
摘要： Urea Selective Catalytic Reduction (urea SCR) system is widely used for diesel engine to reduce the emission of NOx by NH3 which is provided by a hydrolysis of urea water. Concentration distribution of NH3 in an exhaust pipe is an important factor for improvement of the SCR efficiency and prevention of NH3 slip and urea deposit. Therefore, it is necessary to measure two-dimensional (2D) concentration of NH3 in detail. The purpose of this study is to develop the real-time two cross-sectional measurements technology of NH3 concentration using the computed tomography-tunable diode laser absorption spectroscopy (CT-TDLAS). Theoretical NH3 concentration distribution which was reconstructed by CT agreed to CFD results and quadruple pipe’s results showed good resolution by 14th order reconstruction. Therefore, this method has enough resolution and accuracy for measuring the concentration distribution of NH3. And this method was employed in a bent pipe model demonstrated a urea SCR system. The experimental results of two cross-sectional 2D concentration of NH3 show differences of the concentration distribution of NH3 each cross-section and flow pattern like swirl flow. It was found that CT-TDLAS was an effective method to measure concentration distribution of NH3 and observe characteristics of flow. In addition, observing flow pattern enable to validate CFD results, and it helps to improve efficiency of after treatment system.
关键词： Urea selective catalytic reduction,NH3 concentration measurement,Exhaust aftertreatment,CT tunable diode laser absorption spectroscopy,Measurement and instrumentation
更新于2025-09-11 14:15:04