研究目的
Investigating the therapeutic effects of a specific herbal medicine on a particular disease.
研究成果
In conclusion, we reported the successful synthesis of the Ni2+ ions doped CsPbClxBr3-x PQDs at room temperature by the modified supersaturated reprecipitation method, in which the different amount of NiCl2 solution was introduced in the reaction medium. The advantage of this synthesis method lies in the fact that it not only efficiently tuned the bandgap of the CsPbClxBr3-x PQDs, from green (508 nm) to blue (432 nm) spectral region is realized, but also the halide vacancy associated to the non-radiative transition of extiton in the PQDs can be efficiently modified. Therefore, the high efficient photoluminescence with PLQY of 89% for the blue emission at 470 nm is achieved in the 2.5% Ni2+ ions doped CsPbCl0.99Br2.01 PQDs, which is the highest result for the CsPbX3 PQDs with blue emission that fulfilling the NTSC standards. Furthermore, the valence band is modulated in the Ni2+ ions doped CsPbClxBr3-x PQDs, leading the elimination of the carrier injection in the LED device, which result in the device with a high luminance of 612 Cd/m2 and a peak EQE of 2.4%. Both of these factors are higher than the current reported best-performing LED based on the blue emitting PQDs, and demonstrate a promising prospect in the LED display applications.
研究不足
The technical and application constraints of the experiments, as well as potential areas for optimization.